VOL. 11, NO. 20, OCTOBER 2016 ISSN 1819-6608
ARPN Journal of Engineering and Applied Sciences
© 2006-2016 Asian Research Publishing Network (ARPN). All rights reserved.
www.arpnjournals.com
12058
CONDENSATION RATE EFFECT ON TOP OF LINE CORROSION IN CO2
ENVIRONMENT
Syuhaidah Bt Saufi Anuar, Mokhtar Che Ismail, Pandian Bothi Raja and Noor A’in Binti A. Rahman
Department of Mechanical Engineering, Universiti Teknologi Petronas, Bandar Seri Iskandar, Perak, Malaysia
E-Mail: syuhaidahsaufi@gmail.com
ABSTRACT
This research focuses on the effect of condensation rate on top of line corrosion (TLC) for carbon steel (X65) in
CO2 environment. The experiment was conducted in a modified glass cell which simulates the TLC phenomena with tested
temperature ranging from 25 °C to 55 °C and the cooling temperature was 7 °C. The corrosion rate was measured by the
weight loss method and the surface morphology was examined by Scanning Electron Microscopy (SEM) coupled with
Energy Dispersive X-ray (EDX). A baseline CO2 corrosion test was also measured simultaneously. The corrosion rate
recorded for TLC was in the range from 0.76 mm/year to 1.53 mm/year. Further, the results evident that increase in
condensation rate, reduces the corrosion rate which relatively lower than bottom line corrosion rate. The formation of Iron
carbonate (FeCO3), which acts as a protective layer is not fully formed and pitting was observed on the surface of the
sample. In conclusion, the modified glass cell of TLC experiment was successfully done and it is found that corrosion rate
increases with the water condensation rate.
Keywords: top of line corrosion, temperature, corrosion rate, carbon steel, CO2, condensation rate.
INTRODUCTION
Top of Line (TLC) corrosion is an important
phenomenon in the oil and gas production industries
worldwide and it is particularly prevalent in a number of
offshore and onshore operations in Asia Pacific. Regional
operators that have experienced TLC corrosion failures or
damage or those that are considering its effects on the
design stage include Chevron Thailand, Chevron Australia
(Gorgon), PTTEP, Total Indonesia, ExxonMobil Malaysia,
Shell Sarawak, Tallisman Malaysia, and others [1].
TLC corrosion occurred because of heat
exchange between the pipe and colder surrounding which
will lead to condensation at the internal upper pipe walls.
The condensed water is low in pH, but highly saturated
and supersaturated with corrosion products which will
increase the pH and formation of iron carbonate will occur
[2]. Most of the condensed water drains to the bottom of
the pipe due to gravity forces. Continuous injection of
inhibitors only can be done at the bottom of the pipe, but
not the top and sides which will expose them to a very
corrosive environment [3]. The condensed water at the top
of line become very aggressive since it combines with
carbon dioxide (CO2) and/ Acetic acid (HAc) to form
acidic gases. Due to various factors, rate and mechanism
of TLC cannot be predicted precisely.
Some factors that influence TLC corrosion due to
CO2 are the temperature of the gas, the temperature of the
pipe wall, the total pressure of the system, the partial
pressure of CO2, the gas velocity and the condensation rate
which affect the corrosion rate in a complex way [3-6].
In 1991, Gunaltun proposed that the iron
concentration in the condensed water dilutes due to the
continuous condensation on the existing droplet at the top
of line. Failure of applied empirical models in his field
cases regarding corrosion prediction made him realized
that the prediction of the critical condensation rate is more
important than the corrosion [7]. However, he did not
mention on how to determine the critical condensation
rate. Gunaltun and Larrey concluded that the critical
condensation rate lies between 0.15 ml.s/m
2
and 0.25
ml.s/m
2
[8]. Gunaltun emphasizes the importance of
studying the condensation rate is essential to TLC
corrosion rate. Zhang. Z and his co-workers [7] were
studied few parameters that affecting the top of line
corrosion such as the effect of temperature and
condensation rate on the iron carbonate film. They thought
that temperature is one of the important parameters as the
protectiveness of the film formed depends on the
temperature. While, they found that the protective film
was very protective at temperatures greater than 70 ºC.
They believed that supersaturation occurs because the
condensation rate is too low to remove the ion produced
quickly [7]. Besides that, they investigate the effect of gas
velocity on TLC and the result is that the corrosion rate
increased as the gas velocity increased as well as the
condensation rate. However, they did not propose any
correlation between the parameters and the corrosion rate
and their experimental result is still questionable. Since
TLC is one of the most challenging corrosion problems in
oil and gas industry, the established TLC mechanism was
modelled by several researchers [9-13]. Singer. M. et. al
[4] were successfully measured the corrosion rate of the
iron sample at a gas temperature of 40 °C and found that
the general corrosion rate remains constant at a fairly low
value throughout the test compared to the gas temperature
of 70 °C. This study is focusing on the effect of
condensation rate at controlling temperature from 40 °C
to 55 °C, in order to study the properties of film forming
and the TLC behavior at low temperature in a modified
glass cell by weight loss method. The TLC at ambient
temperature also was done for a comparison purpose.
Furthermore, the corrosion rate of the bottom of line
corrosion also was monitored for a baseline test.