A.Azhagu Parvathi et al./ Elixir Condensed Matter Phys. 60 (2013) 16407-16419 16407
1.Introduction
Present decade is witnessing a tremendous improvement in the study of optical and electro-optical properties in
the low dimensional semiconductor systems due to the invention of novel experimental techniques. Nano-semiconductors
with the desired sizes are manufactured out of these techniques. Spherical semiconductor nanocrystals with the diameter
ranging between 1nm and 5nm are synthesized using some simple experimental methods such as wet chemical approach.
Moreover, these low dimensional semiconductor nanostructures depend on the energy spectrum of a confined exciton in
order to bring out the exotic behaviour of the physical properties with the effect of quantum confinement. These unique
properties are used for biological imaging and sensing and may replace the conventional fluorophores with the multiple
fluorescence emission [1]. The quantized energies as well as the motion of the exciton will lead a widening band gap if
the radius of the nanocrystal smaller than the exitonic Bohr radius [2,3]. The reports in this emerging field direct us to
produce novel materials involving some potential applications especially in non-linear opto-electronic devices for
controlling the optical signals in optical computers [4,5].
Semiconductor nanocrystals especially II-VI compound nanoparticles will have a large number of potential
applications such as photovoltaic cells and luminescent materials [6,7] due to its tunable band gap if the impurities are
introduced with the appropriate proportion. The CdS/Zn
x
Cd
1-x
S quantum dot has a large lattice mismatch between the
well and barrier layers. So it is important to include the effect of biaxial strain induced by the lattice mismatch which
eliminates the degeneracy of the top of valence band. Spontaneous and piezoelectric polarizations, generating built-in
electrostatic field especially in wurtzite heterostructures, determine the quantum states of excitons in a quantum dot.
Zn
x
Cd
1-x
S is a direct band gap material, and its band gap varies with the range 2.5 eV- 3.5 eV, a promising candidate for
light emitting diodes with visible emissions with the proper introduction of Cd content. Hence it becomes more important
to understand the excitonic recombination and the band alignment of CdS /Zn
x
Cd
1-x
S compounds. A larger exciton
Interband absorption coefficients in a strained Zn
0.2
Cd
0.8
S/ZnS quantum dot
A.Azhagu Parvathi
1
and A.John Peter
2*
1
Department of Physics, VV Vanniaperumal College for Women, Virudhunagar-626 001.India.
2
Department of Physics, Govt.Arts and Science College, Melur-625 106. Madurai, India.
ABSTRACT
Interband optical absorption coefficients in a strained Zn
0.2
Cd
0.8
S/ZnS quantum dot are
discussed theoretically taking into account the internal field induced by the spontaneous and
piezoelectric polarizations. The effects of geometrical quantum confinement on the exciton
binding energies in Zn
x
Cd
1-x
S/ZnS quantum dot are investigated for various confinement
potentials and thereby the interband optical transition energy associated with the photon is
brought out. The effects of quantum confinement on the heavy hole exciton are brought out
here. We calculate the oscillator strengths for the heavy hole and light hole excitons and the
total nonlinear optical absorption coefficients in a Zn
0.2
Cd
0.8
S /ZnS quantum dot with the
incident photon energy taking into account the effective mass anisotropy of holes. Our
results bring out that the oscillator strength depends on the geometrical confinement,
electron and hole wave functions and the interaction between them, and the nonlinear optical
absorption coefficient shows larger values for smaller dots.
© 2013 Elixir All rights reserved.
ARTICLE INFO
Article history:
Received: 23 May 2013;
Received in revised form:
24 June 2013;
Accepted: 12 July 2013;
Keywords
Exciton binding energy,
Piezoelectricity and spontaneous
polarization,
Quantum dot.
Elixir Condensed Matter Phys. 60 (2013) 16407-16419
Condensed Matter Physics
Available online at www.elixirpublishers.com (Elixir International Journal)
Tele: +91 9786141966
E-mail addresses: a.john.peter@gmail.com
© 2013 Elixir All rights reserved