ISSN 1995-0780, Nanotechnologies in Russia, 2010, Vol. 5, Nos. 11–12, pp. 844–850. © Pleiades Publishing, Ltd., 2010.
Original Russian Text © M.M. Galagudza, D.V. Korolev, D.L. Sonin, I.V. Aleksandrov, V.N. Postnov, G.V. Papayan, E.V. Shlyakhto, 2010, published in Rossiiskie nanotekhnologii,
2010, Vol. 5, Nos. 11–12.
844
INTRODUCTION
The concept of targeted drug delivery implies the
selective accumulation of drugs in pathologically
changed tissue after the systemic introduction of a
complex “drug carrier” with a minimal effect on intact
organs and tissues from the drug [1]. The idea of tar-
geted delivery was first suggested by Paul Ehrlich in
1906 when he introduced the notion of a “magic bul-
let” oriented only against target cells with no influence
on healthy tissue [2]. In contemporary medical prac-
tice, most drugs are applied orally or parenterally,
which is accompanied by their natural biodistribution
and systemic effect on the organism. It is evident that,
in focal pathological processes such as tumor growth,
inflammation, and ischemia, a local increase in drug
concentration in the pathological zone is more attrac-
tive from a clinical point of view; it makes it possible to
decrease the toxicity of many preparations and simul-
taneously achieve a better therapeutic effect.
The use of nanoparticles for the transportation of
drugs makes it possible to achieve the targeted delivery
of the latter in disturbed tissue, as well as increase the
stability of many preparations and their salvation in
water. Two variants of targeted delivery with the use of
nanoparticles are singled out: passive and active trans-
fer. Passive transfer was first described in 1986 when
the selective accumulation of drug conjugates in the
tumor tissues of mice was revealed [3]. This phenom-
enon was called “effect of hypermeability and reten-
tion.” Thus, passive transfer is based on the preferen-
tial exiting of nanoparticles in the damaged area as a
result of the increased meability of vessels of the tumor
microvasculature. Active transfer implies the attach-
ment of so-called directing ligands to the surface of
transport nanoparticles, which provides a highly spe-
cific connection of nanoparticles to the damage
marker on the target cells. Monoclonal antibodies and
their antigen-recognition enzymes, aptamers, and
low-molecular compounds (folic acid, for example)
are most often used as directing ligands. A typical nan-
otransporter for the targeted delivery of drugs consists
of several functional elements, namely, a carrier nano-
particle with an immobilized drug that directs the
ligand in the case of an active transfer and a radioactive
or fluorescent label that makes it possible to the assess
the biodistribution of nanoparticles in the organism.
Until now, studies of the targeted delivery of drugs
were mainly concentrated in oncology. However, it
could be supposed that the concept of targeted drug
delivery may be effectively applied in all local patho-
logical processes, including ischemic reperfusion and
inflammation. Ischemic heart disease is presently the
main cause of death in the world, and it is predicted
the situation will not change until 2020 [4]. This is why
decreasing the after effects of the ischemic reperfusion
of myocardium is one the most important tasks of con-
temporary medical science. The targeted delivery of
cardioprotective drugs (angiogenic growth factors,
recombinant erythropoietin, activators of ATP-sensi-
tive potassium channels, etc.) able to bind with nan-
otransporters covalently or noncovalently may be one
Passive Targeting of Ischemic Myocardium
with the Use of Silica Nanoparticles
M. M. Galagudza
a, b
, D. V. Korolev
a, b
, D. L. Sonin
a, b
, I. V. Aleksandrov
a
,
V. N. Postnov
a, c
, G. V. Papayan
a, b
, and E. V. Shlyakhto
a, b
a
Almazov Federal Heart, Blood and Endocrinology Center, St. Petersburg, ul. Akkuratova 2, 197341
b
Pavlov State Medical University, St. Petersburg, ul. L’va Tolstogo 6/8, 197022
c
Faculty of Chemistry, St. Petersburg State University, St. Petersburg, Universitetskaya nab. 7–9, 199034
e-mail: galagoudza@mail.ru
Received June 13, 2010
Abstract—The clinical outcome in patients with ischemic heart disease can be significantly improved with
the implementation of targeted drug delivery directly into the ischemic myocardium. In this study we describe
the concept of heart-targeted drug delivery with the use of silica nannocarriers. The techniques of nanopar-
ticle functionalization, as well as the data on the effects that silica nanoparticle formulations have on the
parameters of systemic hemodynamics, are also presented. The natural biodistribution of fluorescein- and
indocyanine green-labeled silica nanoparticles was studied with the use of optical fluorescence. We showed
in the study that silica nanoparticles accumulated in the ischemic-reperfused area of the heart, thus providing
the first experimental evidence for passive heart targeting. In conclusion, silica nanoparticles are prospective
drug carriers that have no toxic effect during acute intravenous administration.
DOI: 10.1134/S1995078010110145
ARTICLES