Modelling of the ultrasonic disintegration of activated sludge
N. Lambert*, I. Smets**, J. Van Impe**, R. Dewil*
*KU Leuven, Department of Chemical Engineering, Process and Environmental Technology Lab, Jan Pieter De Nayerlaan 5 –
BE-2860 Sint-Katelijne-Waver - Belgium
(e-mail: nico.lambert@cit.kuleuven.be).
**KU Leuven, Department of Chemical Engineering, Chemical and Biochemical Process Technology and Control Division –
W. de Croylaan 46 – BE-3001 Heverlee - Belgium (e-mail:ilse.smets@cit.kuleuven.be)
Abstract: Ultrasonic treatment of waste activated sludge is one of the possibilities to reduce excess
sludge production through the mechanism of sludge disintegration and cell lysis. In the past, several
attempts have been made to model the process of solubilisation of the particulate volatile suspended solid
part of the activated sludge (VSS) into soluble COD (sCOD). However, the focus of these models was
predominantly on predicting an efficiency factor for the release of sCOD (Disintegration Degree, DD
COD
)
and provided no information on the release of nutrients and the instantaneous reduction of VSS.
Moreover, often insufficient influential variables were included in the model equations, making the
models only applicable on the training dataset of their own experimental research. This paper, therefore,
seeks to build a simple model, which contains all influential input variables, that can predict not only the
sCOD release but also the nutrients release (ortho-PO
4
-P and soluble Kjeldahl nitrogen) and VSS
reduction simultaneously. Therefore, in first instance, a Principal Component Analysis (PCA) is carried
out on the input and output data matrix of obtained experimental observations that will be used as
training data. In this way, certain correlated input variables and independent output variables can be
removed from the model, in order to increase its simplicity and predictive nature. Then, the model is built
on the basis of Partial Least Squares Regression (PLS-R) and a part of the observations is used to validate
the predictive strength of the model.
Keywords: wastewater treatment modelling, ultrasonic disintegration, excess activated sludge reduction.
1. INTRODUCTION
Focused on considerably reducing the generation of excess
sludge in activated sludge wastewater treatment plants, cell
lysis and cryptic growth of microorganisms has been found
very effective to reduce Waste Activated Sludge (WAS).
Ultrasonication of WAS and RAS (Return Activated Sludge)
is capable of destroying the flocs within their matrix of
extracellular polymeric substances (EPS) to result first in
much smaller flocs and afterwards in cell death and lysis
(Xiaoxia Wang, 2010). Cell lysis is a process in which the
cell disintegrates after which the organic, nitrogen and
phosphorus constituents of the cell provide an autochthonous
substrate that contributes to the organic loading of the
wastewater. Growth on such lysis products is described as
cryptic growth and results in a reduced overall biomass
production (Low and Chase, 1999). In most of the scientific
publications on the topic of ultrasonic sludge disintegration
the efficiency of the process is assessed by the release of
sCOD in the supernatant liquid of the activated sludge. It is
assumed that the solubilisation of particular COD (pCOD)
into soluble COD (sCOD) involves first deagglomeration of
the active sludge flocs (floc disintegration), and, second, the
release of the cellular material in the supernatant liquid as a
result of the breakage of the cell wall (cell lysis) (Si-Kyun et
al.). However, in current literature little attention is given to
the release of nitrogen and phosphorous compounds in the
supernatant liquid during the process of sludge disintegration
although, e.g., Bougrier et al. (2005) highlight that nitrogen is
mainly released as proteins and amino acids and that, at
moderate specific energies, a solubilisation degree of 40%
can be expected. Several previous research papers reported
relevant models for single alkaline activated sludge
treatment, single ultrasonic sludge disintegration and the
combined treatment process (e.g., Li et al., 2010; Wang et al.,
2005 and Kim et al., 2010). All these models use a different
combination of independent predictive variables to determine
the sCOD release in the supernatant liquid of the activated
sludge. It is evident that there are still a lot of questions that
remain unanswered. In the first place, it can be said that the
choice of the appropriate predictor variables to describe the
untreated activated sludge itself and to characterize the
process conditions of the ultrasonic sludge treatment is of
great importance to generate an appropriate ultrasonic sludge
disintegration model. For example, it seems logical to
characterize the treated sludge on the basis of both the initial
(biomass quantity related) MLSS
0
and MLVSS
0
concentration. In this way it will be taken into account
whether or not we are dealing with a more organic or more
inorganic activated sludge or whether the sludge sample is
highly thickened or not. The ultrasonic reactor design can be
described by the ultrasonic density (D
S
- W/cm
2
) and the type
of ultrasonic horn or transducer can be quantified by the
ultrasonic intensity (I
S
– W/mL). To have a global view on
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