Anisotropic optical conductivity of Sr 3 Ru 2 O 7 C. Mirri, 1 L. Baldassarre, 1 S. Lupi, 1 M. Ortolani, 2 R. Fittipaldi, 3 A. Vecchione, 3 and P. Calvani 1 1 Dipartimento di Fisica and CNR-INFM “Coherentia,” Università di Roma La Sapienza, Piazzale A. Moro, 2, I-00185 Roma, Italy 2 Berliner Elektronenspeicherring-Gesellschaft für Synchrotronstrahlung m.b.H., Albert-Einstein Strasse 15, D-12489 Berlin, Germany 3 Dipartimento di Fisica “E. R. Caianiello”, Università di Salerno and CNR-INFM Laboratorio Regionale Supermat, Via S. Allende, I-84081 Baronissi Salerno, Italy Received 30 May 2008; published 31 October 2008 The optical conductivity of Sr 3 Ru 2 O 7 has been studied both in the ab planes, between 12 and 450 K, and along the c axis between 12 and 300 K. ab is Drude-type but, for increasing T, it shows a crossover around 300 K to a regime with enhanced scattering rate, probably driven by a stronger coupling with the optical phonons. The spectral weight shows the imprints of strong correlations, but less pronounced than in a high-T c material. Along the c axis, the Drude term has a much smaller plasma frequency, and a strong absorption appears at 1 eV. These findings indicate an anisotropic metallic state where electron-electron and electron-phonon interactions play a major role. This picture may be reconciled with the local-density calcula- tions reported in the literature, which predict an insulating c axis, once those interactions are taken into account. DOI: 10.1103/PhysRevB.78.155132 PACS numbers: 74.70.Pq, 78.30.-j, 78.20.-e I. INTRODUCTION The Ruddlesden-Popper-type series Sr n+1 Ru n O 3n+1 n =1,2, and has attracted wide interest in the last decade due either to the unconventional superconductivity of Sr 2 RuO 4 n =1, where the Cooper pairs are in a p-symmetry triplet state, 1 or to the metamagnetism and quantum critical- ity shown by Sr 3 Ru 2 O 7 n =2at T 1 K. 2,3 In turn, SrRuO 3 n = is the only ferromagnetic material among the itinerant 4d transition-metal oxides. 4 In the present paper we focus on the double-layered, nonsuperconducting, perovskite Sr 3 Ru 2 O 7 , with the aim to investigate its basically unex- plored, anisotropic, optical properties. The interest for aniso- tropic, conducting oxides has grown in recent years after the discovery of high-T c superconductivity in the cuprates, which share with the ruthenates the perovskite structure and the typical transition metal-oxygen layer. Moreover, single crystals, large and pure enough along different axes, have been grown successfully for many chemical compositions, allowing for a detailed determination of their anisotropic be- havior by different spectroscopic techniques. Sr 3 Ru 2 O 7 has a quasitetragonal cell elongated along the c axis. In the calculations of both electronic and phonon bands, a symmetry I4 / mmm is generally assumed. However, under rotations of the RuO 6 octahedra around the c axis, such structure tends to transform into lower-symmetry orthorhom- bic phases like Bbcb no. 68. 5 At room temperature, the average values for the lattice constants of the tetragonal cell are a= a + b/ 2=0.5500 nm with a b, and c =2.0725 nm. At 40 K a = b, and below this temperature a b. 5 The octahedra RuO 6 are formed by the hybridized bonds between the 2p levels of oxygen and the 4d levels of Ru 4+ , which host four electrons. In the crystal field these orbitals are split by an energy 6 10Dq, into a triplet t 2g and a doublet e g . In Sr 3 Ru 2 O 7 , the crystal field is strong enough that 10Dq J, where J is the Hund energy. Therefore, in the ground state the four electrons are in the t 2g state, e g is empty, and the total spin S is 1. In turn, the degeneracy of the t 2g state is removed by the Jahn-Teller distortion. In Sr 3 Ru 2 O 7 the carriers are holes, as shown by Hall data. 7 The resistivity is anisotropic, consistently with the quasi-two-dimensional Fermi surface extracted from band- structure calculations. 8 Indeed, both the ab plane resistivity ab Tand that along c, c T, are metallic. However, at 300 K c T 40 ab T. 9 This latter is linear down to 15 K, while 10 ab TT 1.5 between 15 and 6 K, T 2 below 6 K. This change in slope, which is much more pronounced in c T, corresponds to a peak in the magnetic susceptibility at 16 K which was tentatively interpreted in terms of ferromag- netic fluctuations. 9 A ferromagnetic phase is observed only under external pressure, with a Curie temperature T c 70 K at 1.1 GPa. 11 Concerning the optical properties, those of 12,13 Sr 2 RuO 4 and of 14 SrRuO 3 have been studied in detail, while for Sr 3 Ru 2 O 7 only the room-temperature optical conductivity ab of the ab plane can be found in the literature. 15,16 ab appears metallic in the midinfrared and shows elec- tronic bands above 3 eV, which are attributed to charge- transfer CTtransitions between the O 2p and the Ru t 2g levels. Spectra at lower temperatures were reported only in the region of the stretching mode of the Ru-O bond, to study how its peak frequency depends on T. The present experiment is aimed at completing our optical knowledge of Sr 3 Ru 2 O 7 , by measuring its both with the radiation field polarized in the ab plane between 12 and 450 Kand along the c axis between 12 and 300 K, for ranging from the far infrared to the near UV. II. SAMPLE AND EXPERIMENT The Sr 3 Ru 2 O 7 single crystal was grown by the floating zone technique and characterized by x-ray diffraction and scanning electron microscopy. Traces of the Sr 4 Ru 3 O 10 phase, as usual in these samples, were found. The reflectivity Rof the crystal was measured at nearly normal incidence PHYSICAL REVIEW B 78, 155132 2008 1098-0121/2008/7815/1551326©2008 The American Physical Society 155132-1