Materials Sciences and Applications, 2021, 12, 315-329
https://www.scirp.org/journal/msa
ISSN Online: 2153-1188
ISSN Print: 2153-117X
DOI: 10.4236/msa.2021.127021 Jul. 2, 2021 315 Materials Sciences and Applications
A Comparison of Optical Properties of CuO and
Cu
2
O Thin Films for Solar Cell Applications
Radu Bunea, Ashwin Kumar Saikumar, Kalpathy Sundaram
University of Central Florida, Orlando, USA
Abstract
Solar energy is becoming more popular and widespread, and consequently,
the materials to manufacture solar cells are becoming more limited and cost-
ly. Therefore, in order to keep solar energy affordable and available, we must
research alternative materials such as copper oxides. Some benefits of copper
oxides include being available in abundance, affordable, low toxicity, low
bandgap, and a high absorption coefficient—all of which contribute to it be-
ing a valuable interest for the manufacturing of solar cells. In this study, CuO
thin films were synthesized utilizing RF sputtering technique with deposition
occurring at room temperature followed by thermal annealing between 100˚C
and 400˚C and using different gases, oxygen (O
2
) (oxidizing and reactive gas)
and nitrogen (N
2
) (inert gas), besides air. Afterwards, these thin films were
evaluated for a range of wavelengths: 200 - 400 nm (UV spectrum), 400 - 700
nm (Visible spectrum), and 700 - 800 nm (IR spectrum), for both, optical
transmittance and photoluminescence. In addition, the CuO results were com-
pared to our Cu
2
O results from a previous study to assess their differences. In
the results of this study, the CuO thin film initially had a bandgap of 2.19 eV
at room temperature, and by increasing the annealing temperature to differ-
ent levels, the bandgap decreased respectively. The presence of air in the
chamber allowed for the highest decrease, followed by the nitrogen (N
2
) and
the lowest decrease was observed in the presence of oxygen (O
2
). This was re-
flected in the decrease in the bandgap values from 2.19 eV (room tempera-
ture) to 2.05 eV for the films annealed at 400˚C.
Keywords
Cu
2
O Thin Film, Cuo Thin Film, Optical Properties, Bandgap, Photoluminescence
1. Introduction
The current materials used to manufacture photovoltaics are becoming scarce,
How to cite this paper: Bunea, R., Saiku-
mar, A.K. and Sundaram, K. (2021) A Com-
parison of Optical Properties of CuO and
Cu
2
O Thin Films for Solar Cell Applica-
tions. Materials Sciences and Applications,
12, 315-329.
https://doi.org/10.4236/msa.2021.127021
Received: May 5, 2021
Accepted: June 29, 2021
Published: July 2, 2021
Copyright © 2021 by author(s) and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access