Hindawi Publishing Corporation
ISRN Physical Chemistry
Volume 2013, Article ID 547378, 7 pages
http://dx.doi.org/10.1155/2013/547378
Research Article
Influence of Surfactants and Dissolved Gases on
the Silver Nanoparticle Plasmon Resonance Absorption Spectra
Formed by the Laser Ablation Processes
Ming Jing Chua
1
and Yoshinori Murakami
2
1
Department of Materials Science, Nagaoka National College of Technology, Nagaoka, Niigata 940-2188, Japan
2
Department of General Science, Hachinohe National College of Technology, Hachinohe, Aomori 039-1104, Japan
Correspondence should be addressed to Yoshinori Murakami; murakami-g@hachinohe-ct.ac.jp
Received 10 April 2013; Accepted 15 May 2013
Academic Editors: D. Knopf, T. Panczyk, and S. Sasaki
Copyright © 2013 M. J. Chua and Y. Murakami. Tis is an open access article distributed under the Creative Commons Attribution
License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly
cited.
Te silver nanoparticles were fabricated by the focused laser irradiation to silver rod immersed in various kinds of surfactant
aqueous solutions. It was found that anionic and cationic surfactants showed diferent roles on the silver nanoparticle growth
during the focused laser irradiation processes. Silver nanoparticle synthesis in an amphoteric surfactant aqueous solution was also
carried out using the same techniques, and it was found that the spectral shifs for these surface plasmon bands showed complicated
behaviors against the concentration of amphoteric surfactants as well as pH. Furthermore, the infuence of the gas dissolved in a
solution on the silver nanoparticle growth during the focused laser irradiation processes was investigated. With increasing the gas
pressure of CO
2
, the surface plasmon bands of silver nanoparticles were shifed to longer wavelength, suggesting that the dissolved
gas of CO
2
in a solution enhances the silver nanoparticle growth. Te plausible mechanism was proposed to understand the reason
of such enhancement of silver nanoparticle growth by increasing the dissolved gas in a solution.
1. Introduction
Nanoscale materials have attracted much attention due to
their unique properties being diferent from their bulk mat-
erials [1]. For example, gold and silver nanoparticles have
been used in various analytical techniques such as catalysis,
biosensing, recording media, and photoscience. From the
production point of view, chemical reduction of metal ions
is mostly commonly employed in the preparation of metal
nanoparticles in solution. In the last few years, a new metho-
dology based on the laser ablation of bulk metal in water
appeared for generating metal nanoparticles. Te use of sur-
factants, especially, which covers the particles during their
condensation, promotes improved size uniformity as well as
reduces the coalescence during the fabrication of nanopar-
ticles using such laser ablation techniques. Mafun´ e et al.
[2] reported for the frst time that the size distribution of
silver nanoparticles produced by the laser ablation varied
with the addition of sodium dodecyl sulfate (denoted by
SDS hereafer) in water, and they also reported that the size
became smaller and narrower with increasing the concen-
tration of SDS. Te authors also attempted the formation
of stable platinum nanoparticles using the laser ablation of
platinum plate in water and found that the particle diameter
of platinum nanoparticles decreased with increasing the
concentration of SDS [3]. Although the efects of the anionic
surfactants of SDS on the size distribution of the laser ablated
metal nanoparticles have been thoroughly investigated, very
few works have been done for the infuences on the other
anionic and cationic surfactants.
As an example of the investigations on the infuence of
a cationic surfactants, Chen and Yeh [4] have investigated
the particle diameters of silver nanoparticles formed by the
laser ablation of silver rod from the enlarged transmission
electron photographs and found that the particle diameters
were 4.2 nm and 7.8 nm with the addition of the anionic SDS
and the cationic cetyltrimethylammonium bromide (denoted
by CTAB hereafer), respectively. Tey concluded that the