224 Journal of Non-Crystalhne Solids 126 (1990) 224-230
North-Holland
Raman study of lead borate glasses
B.N. Meera, A.K. Sood, N. Chandrabhas and J. Ramakrishna 1
Department of Physws, In&an Insutute of Scwnce, Bangalore- 560 012, Indta
Received 9 November 1989
Revised manuscript received 18 July 1990
Glasses in the system xPbO:(100- x)B203 (22 _<x < 85 mol%) have been studied by Raman spectroscopy with a view to
understand the effect of PbO on the borate network. The conversion of three-fold to four-fold coordinated boron takes place
primanly by incorporation of BO4 into boroxol rings in the form of pentaborate and diborate umts. For high lead content,
back conversmn of four to three coordinatmn of borons occurs and the network consists primardy of pyroborate, orthoborate
and metaborate groups.
1. Introduction
Raman spectroscopy has proved to be a useful
tool in the study of amorphous materials. Raman
spectra of crystalline and vitreous borates have
been used as a basis for the qualitative identifica-
tion of glass forming structural units in these
glasses [1-3]. Due to structural disorder a com-
plete vibrational analysis in glasses is not possible
from an ab-initio point of view and an analysis is
done primarily by comparing the spectra of these
glasses with those of crystalline borates for which
the structures are known.
Pure B203 and alkali borate glasses, R20-B203
(R = Li, Na, K, Cs and Rb), have been studied
extensively by Raman scattering [4-16]. Pure
vitreous B203 is known to be made up of a ran-
dom network of boroxol rings in which borons are
three coordinated [17]. The addition of alkali oxide
results in the formation of four coordinated
borons, and the fraction of these four coordinated
units can be estimated by NMR [18-22]. By com-
bining the Raman scattering studies and NMR
investigations with the available crystallographic
data, structural groups present in these glasses
i Author to whom correspondence should be addressed.
have been clearly identified. Figure 1 shows the
several structural groups present in various borate
compounds.
Lead borate, xPbO : (100 - x)B203, is an inter-
esting system because the glass phase can be
formed over a wide concentration of lead oxide
[23,24]. Moreover, PbO can enter the glass net-
work both as a network modifier and also as a
network former. Hence the structure of these
glasses is expected to be different from that of
alkali borate glasses. Bray and co-workers [25,26]
have carried out NMR investigations of lead
borate glasses and compounds and their study
indicates that N 4 (the fraction of the four coordi-
nated boron atoms in the glass) increases with the
PbO content up to 50 mol% PbO. Further increase
of PbO decreases the value of N 4. Not much
Raman spectroscopic work has been carried out
on lead borate glasses with the exception of the
preliminary work of Konijnendijk and Verweij
[27], in which the spectra of xPbO : (100 - x)B203
for x = 25, 33.3, 50 and 70 mol% are presented.
The peak assignment and the identification of the
structural groups have not been completely made.
Therefore, the present work consists of a sys-
tematic study of the xPbO :(100- x)B20 3 glass
system covering a wide range of concentration
with x varying between 22 and 85 mol%.
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