Research Article Adv. Mater. Lett. 2015, 6(2), 104-113 ADVANCED MATERIALS Letters
Adv. Mater. Lett. 2015, 6(2), 104-113 Copyright © 2015 VBRI Press
www.amlett.com, www.vbripress.com/aml, DOI: 10.5185/amlett.2015.5612 Published online by the VBRI press in 2015
Solvent free, efficient, industrially viable, fast
dispersion process based amine modified
MWCNT reinforced epoxy composites of
superior mechanical properties
Bhanu Pratap Singh
1*
, Veena Choudhary
2
, Satish Teotia
1
, Tejendra Kumar Gupta
1
, Vidya Nand
Singh
3
, Sanjay Rangnath Dhakate
1
, Rakesh Behari Mathur
1
1
Physics and Engineering of Carbon, Division of Materials Physics and Engineering, CSIR-National Physical Laboratory,
New Delhi 12, India
2
Centre for Polymer Science and Engineering, Indian Institute of Technology Delhi, Delhi 16, India
3
Electron Microscopy Section, CSIR-National Physical Laboratory, New Delhi 12, India
*
Corresponding author. Tel: (+91) 11 45608460; E-mail: bps@nplindia.org
Received: 12 August 2014, Revised: 03 November 2014 and Accepted: 15 November 2014
ABSTRACT
Dispersion of multiwalled carbon nanotubes (MWCNTs) into epoxy resin is a challenging task for the process to be viable on
industrial scale. Herein, amine functionalized MWCNTs (Am-MWCNTs) were reinforced into epoxy resin using industrially
viable, fast, efficient, solvent free, high speed homogenizer dispersion technique. Am-MWCNTs ranging from 0.1 to 0.75% by
w/w were loaded in epoxy and the effects of loading of Am-MWCNTs on mechanical properties of epoxy composites are
investigated. The flexural strength of Am-MWCNTs based epoxy composites reached up to 163 MPa for 0.5 wt% MWCNTs
loaded sample compared to 95 MPa for pure cured epoxy sample; an overall improvement of 72% in the flexural strength. In
addition to this, the flexural modulus value reached to 3795 MPa for 0.75 wt% Am-MWCNTs loaded sample from 2250 MPa
for pure epoxy sample, an improvement of 69%. The enhancement in the mechanical properties was correlated with the
dynamic scanning calorimeter results, TEM and SEM images of fractured surface. The substantial improvement in the
mechanical properties of the epoxy resin at such low CNT loading can open a venue for the preparation of structurally strong
structures for aerospace, defence, automobile and sports industries. Copyright © 2015 VBRI Press.
Keywords: Multiwalled carbon nanotubes; functionalization; mechanical properties; dispersion; high speed homogenizer.
Bhanu Pratap Singh is a Senior Scientist at
CSIR-National Physical Laboratory, New
Delhi, India. He did B.Tech in Chemical
Engineering from I.E.T. Lucknow, India,
M.Tech in Chemical Engineering from IIT
Kanpur, India and PhD form IIT Delhi, India.
He has more than 10 years of research
experience in the field of synthesis of carbon
nanomaterials and their composites for
structural, EMI shielding and anodes of Li-ion
Batteries applications. He has published more
than 50 research articles in reputed journals, 3 patents and author of three
contributory chapters in international books. He is the editor of four
international journals.
Veena Choudhary is a well known
distinguished professor in the field of Polymer
Science and Engineering. Presently she is
occupying the position of Reliance Chair
Professor and Head, of Centre for Polymer
Science and Engineering at IIT Delhi. She
obtained her Ph.D. from IIT, Delhi in 1977. She
has published/ presented more than 270 papers
in Journals /conferences and five patents to her credit. She is a recipient
of very prestigious awards from Germany-Alexander Von Humboldt
Fellow during 1985-86, Indo-US Science and Technology Fellow USA
during 1992-93 and visiting Professor in the University of Lund, Sweden,
during 2000-2001.
R.B. Mathur is presently associated as
Emeritus Scientist at the CSIR-National
Physical laboratory, New-Delhi, India. He
specializes in Advanced carbon products e.g.
carbon fibres; CNTs, carbon fibre and CNT
reinforced polymer and carbon-carbon
composites, carbon materials for energy
applications etc. He has Published 152
research papers in peer reviewed journals, 4
chapters in books, applied/granted 13 patents,
and transferred 5 technologies to industries.
He has been a recipient of NRDC award (1993), CSIR-Raman Research
Fellowship (1999), CSIR-Process Technology Shield (1999), B.D. Bangur
Award (2006), Endeavour India Executive award from Govt. of Australia
(2007).