BASIC INVESTIGATION Impact of Iontophoresis and PACK-CXL Corneal Concentrations of Antifungals in an In Vivo Model Ayse Kalkanci, MD, PhD,* Nilufer Yesilirmak, MD,Hüseyin Baran Ozdemir, MD, Elif Ayca Unal, MD,* Merve Erdogan, PhD,* Tamay Seker, PhD,§ Atakan Emre Tum, MS,¶ Ahmet Kamil Karakus, MS,¶ Kenan Hizel, MD,k and Kamil Bilgihan, MD** Purpose: To investigate voriconazole (VRZ) penetration and fungal load in the cornea after applying VRZ therapy with various treatment combinations in a fungal keratitis model. Methods: Fifty-four eyes of 27 young albino rabbits were provided for this experimental study. Twelve corneas were inoculated with Candida albicans, 12 corneas were inoculated with Fusarium solani, and 6 eyes were selected as controls. Infected corneas received various treatment combinations including VRZ 1% drop therapy alone, VRZ 1% plus amphotericin B 1% drop combination therapy, iontophoretic VRZ therapy, and VRZ 1% drop therapy after corneal cross-linking. Fungal load was measured by log reduction, and VRZ levels were quantied by liquid chromatographytandem mass spectrometry. Results: Iontophoresis-assisted VRZ application showed the high- est antifungal activity against F. solani keratitis (4-log reduction) and C. albicans keratitis (5-log reduction) compared with other treatment applications. VRZ levels were also found to be the highest in corneas that received iontophoretic VRZ treatment (3.6313 6 0.0990 ppb for F.solani keratitis and 1.7001 6 0.0065 ppb for C. albicans keratitis) compared with other treatment applications. Conclusions: Iontophoresis seems to provide the highest VRZ concentration and highest antifungal activity in the cornea compared with other treatment applications for C. albicans and F. solani keratitis. Key Words: keratitis, voriconazole, iontophoresis, corneal cross- linking, liquid chromatography tandem mass spectrometry (Cornea 2018;37:14631467) F ungal keratitis is a serious infection of the cornea that can progress from corneal ulcer to corneal perforation rapidly without proper treatment. 1 The most frequently encountered pathogens are Fusarium spp, Candida albicans, and Asper- gillus spp. 2,3 Most common risk factors for fungal keratitis include ocular trauma, contact lens wear, ocular surgery, immune system deciency, prolonged use of corticosteroids, and other ocular surface diseases. 3 Despite many studies and these known factors, diagnosis of fungal keratitis remains a challenge and the ideal therapeutic regimen is always a matter of debate because of its difculty. 4,5 After reliable and prompt diagnosis of fungal keratitis, the rst and commonly accepted approach is to start appropriate intense medical treatment to prevent sight- threatening complications. 5 There are various antifungal agents 6 in clinical use [such as azoles, natamycin, amphoter- icin B (AMB), etc.], and voriconazole (VRZ: triazole antifungal agent derived from uconazole) is suggested as superior to others in recent years for severe fungal keratitis. 6,7 Application of topical VRZ or other agents often requires hospitalization because of its intensive regimen (hourly use for several days). 8 Still, penetration and absorption of topi- cally applied drugs deep into the cornea are limited because of the corneal barrier function associated with epithelial tight junctions and high electrical resistance. 9,10 Thus, approaches to increase drug absorption such as iontophoresis have attracted great attention. 11,12 Iontophoresis is a technique based on the basic electrical principle that oppositely charged ions attract each other and similarly charged ions repel each another. In this technique, ionized substances are driven into the tissue by electrorepulsion at either the anode for positively charged drugs or the cathode for negative drugs. 13 Ionto- phoresis has been studied for drug delivery in ophthalmol- ogy since 1943. 14 In this noninvasive method, molecules can be transported actively across the cornea or conjunctiva with application of an external electric eld. 13 It has been demonstrated that drugs can be maintained in ocular tissues for hours after iontophoresis, and this drug loading can increase by changing the current density and treatment Received for publication January 30, 2018; revision received May 25, 2018; accepted May 27, 2018. Published online ahead of print August 29, 2018. From the *Department of Medical Microbiology, Gazi University Faculty of Medicine, Ankara, Turkey; Department of Ophthalmology, Yildirim Beyazit University, Ankara, Turkey; Ankara Ulucanlar Eye Training and Research Hospital, University of Health Science, Ankara, Turkey; §Middle East Technical University, Central Laboratory, Molecular Biology-Biotechnology Research and Development Center, Mass Spec- troscopy Laboratory, Ankara, Turkey; ¶Gazi University Faculty of Medicine, Phase 4 Student, Ankara, Turkey; kDepartment of Infectious Diseases, University Faculty of Medicine, Ankara, Turkey; and **Department of Ophthalmology, Gazi University Faculty of Medicine, Ankara, Turkey. This project was supported by an unrestricted grant from Pzer Inc. The authors have no conicts of interest to disclose. Presented as a poster in Trends in Medical Mycology, TIMM; October 69, 2017; Belgrade, Serbia. Correspondence: Ayse Kalkanci, MD, PhD, Department of Medical Microbiology, Gazi University Faculty of Medicine, Ankara, Turkey 06500 (e-mail: aysekalkanci@email.com). Copyright © 2018 Wolters Kluwer Health, Inc. All rights reserved. Cornea Volume 37, Number 11, November 2018 www.corneajrnl.com | 1463 Copyright Ó 201 Wolters Kluwer Health, Inc. Unauthorized reproduction of this article is prohibited. 8