Biosynthesis of Highly Dispersed Palladium Nanoparticles Using Astraglmanna
Aqueous Extract
Khalil Farhadi,
a,
* Atefeh Pourhossein,
a
Mehrdad Forough,
a
Rahim Molaei,
a
Ali Abdi
b
and
Abbas Siyami
c
a
Department of Chemistry, Faculty of Science, Urmia University, Urmia, Iran. P.O.Box 165-5715944931
b
Department of Physics, Faculty of Science, Urmia University, Urmia, Iran
c
University College of Zarrineh, Khoy, Iran
(Received: Jan. 3, 2013; Accepted: Apr. 1, 2013; Published Online: May 16, 2013; DOI: 10.1002/jccs.201300006)
Biosynthesis of nanoparticles has received increased attention due to a growing need to develop environ-
mentally benign technologies in material synthesis and employment of secondary metabolites from plant
extract that has emerged as a novel technology for this purpose. In this study, a rapid and biogenic process
for fabrication of palladium nanoparticles (PdNPs) is reported. Highly dispersed palladium nanoparticles
were successfully prepared by using aqueous extract of Astraglmanna, a non-toxic and eco-friendly mate-
rial, without extra surfactant, capping agent, and template. The PdNPs were characterized by using UV–
Visible spectroscopy, scanning electron microscope - energy dispersive spectra (SEM-EDX), Fourier
transform infra red spectroscopy (FTIR), dynamic light scattering (DLS) and X-ray diffraction (XRD)
analysis. Transmission electron microscopic (TEM) images of the PdNPs were recorded and mean size of
the biosynthesized nanoparticles was found to be approximately 15 nm.
Keywords: Astraglmanna; Biological; Nanoparticles; Palladium; Synthesis.
INTRODUCTION
Nanotechnology applies the techniques and pro-
cesses of micro fabrication to build devices for studying
bio-systems and has a wide range of applications in the va-
riety of fields.
1
Recently, this scientific approach has
emerged as an elementary division of science and technol-
ogy that investigates and regulates the interaction at cell
level between biological and synthetic materials with the
aid of nanoparticles.
2
Nanoparticles of noble and transition
metals, such as gold, silver, platinum, and palladium are
widely used in products that come into direct contact with
the human body including shoes, detergents, cosmetics,
jewelery, and toothpaste, as well as medical, biological and
pharmaceutical applications.
3
To date, there are growing
interests on the research, synthesize and the development
of transition metal nanoparticles owing to their ultra unique
physical, chemical, and thermodynamic properties that
have made them useful in different fields of science, such
as catalysis, medicine, electronics, etc, and for their poten-
tial applications in nanoelectronics. In particular, PdNPs
have become of increasing scientific interest as catalysts
for carbon–carbon bond-forming reactions such as Suzuki–
Miyaura cross-coupling reactions.
4–7
A wide variety of
physical, chemical and biological processes results in the
synthesis of Pd nanoparticles have been reported, some of
these are novel and others are quite common. Moreover,
the usual methods for producing PdNPs involve chemical
reduction of palladium salts aqueous solutions by alcohol,
8
sodium borohydride,
9
hydrazine,
10
poly-ethyleneglycol
(PEG),
11
ascorbic acid,
12
dimethylamine-borane (DMAB)
in supercritical carbon dioxide,
13
and etc. However, there
are evidences for the harmfulness of these synthesized
nanoparticles to the environment and biosystems. Also,
most of these reported methods are extremely expensive
and involve the use of toxic chemicals and hazardous mate-
rials, which may pose potential environmental and biologi-
cal risks. Moreover, these techniques suffer from a certain
complexity and generally require high temperature condi-
tions and special instrumentation to complete the reduction
reaction of soluble palladium ions. Therefore, there is a
need to prepare and employ more and more eco-friendly
nanoparticles that are best suited to environment. Anyway,
exploring the new strategy to manufacturing effective
metal nanoparticles supported with easy and safe prepara-
tion techniques is of great importance for industrial inter-
ests. For these reasons, the synthesis and fabrication of
nanoparticles would benefit from the development of
clean, nontoxic and environmentally acceptable ‘‘green
1144 © 2013 The Chemical Society Located in Taipei & Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim J. Chin. Chem. Soc. 2013, 60, 1144-1149
Article
* Corresponding author. Fax: +98-441-2776707; E-mail: khalil.farhadi@yahoo.com; kh.farhadi@mail.urmia.ac.ir
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