• • * THE JOURNAL or BiOLOGICAL CHEMISTRY ' _ Vol. 263, No. 34, Issue of December 5, pp. 184S9-18465,1988 © 1988 by The American Society for Biochemistry and Molecular Biology, Inc. Printed in U.S.A. Pattern of Protein Phosphorylation in Aortic Endothelial Cells MODULATION BY ADENINE NUCLEOTIDES AND BRADYKININ* (Received for publication, May 11, 1988) Dominique Démolie^, Marc Lecomte, and JeanMarie Boeynaems From the Institute of Interdisciplinary Research, School of Medicine, Free University of Brussels, Campus Erasme, Building C, Route de Lennik 808, 1070 Brussels, Belgium In bovine aortic endothelial cells, ATP (10—100 ^m) and bradykinin (0.11.0 ^M) enhanced the phospho rylation of two major protein substrates with apparent molecular masses of 95 and 28 kDa. The action of ATP involved P2y purinoceptors. The kinetics were distinct for the two phosphopeptides. The phosphorylation of the 95kDa protein was rapid (within 30 s) but tran sient (maintained for only 2 min). This time course agrées with that observed for the increase of the cyto solic Ca^* level induced by ATP in thèse cells. lono phore A23187 (^ 100 nM) induced this phosphorylation for a longer period (510 min), whereas phorbol 12 myristate 13acetate (PMA) was completely inactive. The enhancement of the 28kDa protein phosphoryla tion was détectable after a 5min lag and was main tained for at least 20 min. PMA (50 nM) stimulated weakly the phosphorylation of the 28kDa protein, whereas A23187 (100300 nM) was even more effec tive than ATP and bradykinin. The 95kDa phospho protein seems to be related to a 100kDa substrate of calmodulindependent protein kinase III recently iden tified as elongation factor2. The 28kDa protein, which was resolved as three variants in bidimensional gel electrophoresis, appears very similar to a slightly heavier phosphoprotein from thrombinstimulated hu man platelets. In addition, bidimensional electropho resis allowed the détection of at least 10 substrates (from 18 to 46 kDa) whose phosphorylation was en hanced equally well by ATP, bradykinin, and A23187 and only partially by PMA. In conclusion, protein phos phorylation induced by ATP and bradykinin in aortic endothelial cells seems to be catalyzed mostly by Ca^*- dependent kinases, distinct from protein kinase C. The thromboresistance of the vascular endothelium in volves several mechanisms. One of them is the release of prostacyclin (PGI2)' and nitric oxide: PGI2 and nitric oxide * This work was performed under contract of the "Ministère de la Politique Scientifique" (Action Concertée) and supported by a grant from the "Fonds de la Recherche Scientifique Médicale." The costs of publication of this article were defrayed in part by the payment of page charges. This article must therefore be hereby marked "aduer- tisement" in accordance with 18 U.S.C. Section 1734 solely to indicate this fact. t Supported by the Association de Recherche Biomédicale et de Diagnostic (ARBD). ' The abbreviations used are: PGI2, prostaglandin I2 (prostacyclin); ADP;8S, adenosine 5'0(2thiodiphosphate); ATP7S, adenosine 5' 0(3thiotrisphosphate); APCPP, adenosine 5'(a,/3methylene)tris phosphate; APPNP, adenosine 5'(/3,7imido)triphosphate; BAEC, bovine aortic endothelial cells; Chaps, 3[(3cholamidopro pyl)dimethylammonio]lpropanesulfonic acid; CaM, calmodulin; IP3, inositol (l,4,5)trisphosphate: MEMDVal, minimal essential médium with DvaHne; PAEC: porcine aortic endothelial cells; PGEi, prostaglandin Ei; PMA, phorbol 12myristate 13acetate; SDS, so dium dodecyl sulfate; HUVEC, human umbilical vein endothelial cells. synergize with each other to inhibit the aggregation of plate lets (1), whereas nitric oxide decreases their adhésion to the endothelium (2). Cultured endothelial cells release PGI2 in response to multiple agonists. Human umbilical vein endo thelial cells (HUVEC) are stimulated to synthesize PGI2 after addition of thrombin (3) and histamine (4), whereas ATP and ADP stimulate PGI2 production selectively in aortic endothe lial cells from bovine (BAEC) (5) and porcine (PAEC) (6) origin. Bradykinin, in addition to its stimulatory effect on PGI2 release from BAEC and PAEC (7), stimulâtes the pro duction of nitric oxide by PAEC (8). The action of ADP and ATP might be physiologically relevant. Thèse adenine nucleotides are indeed released dur ing platelet activation, so that they might act as the mediators of a négative feedback loop: they would stimulate the release of PGI2 and nitric oxide from the endothelium adjacent to the thrombus in formation, in order to limit the extent of platelet aggregation. The responses of endothelial cells to ATP seem to be mediated by P2y purinoceptors according to Burnstock's classification (9, 10). One transduction mechanism linked to thèse receptors has been recently identified: the hydrolysis of phosphatidylinositol bisphosphate. ATP induces indeed a rapid and transient increase of the level of inositol (1,4,5) trisphosphate (IP3) (11, 12) and of cytosolic Ca^* (11, 13, 14) in aortic endothelial cells. Bradykinin reproduces thèse effects of ATP in aortic endothelial cells (1518), as do thrombin and histamine in HUVEC (19, 20). In addition, several studies have pointed out the rôle played by protein kinase C in the control of endothelial cells functions. Phorbol 12myristate 13acetate (PMA), a potent activator of protein kinase C which mimics the effect of endogenous diacylglycerol, induces the production of plasminogen activator (tPA) (21), the sécrétion of von Willebrand protein (22), and angiogenesis (23). Our démonstration that PMA and the Ca^* ionophore A23187 act synergistically to stimulate PGI2 production by BAEC (24) seems to indicate a coopération between cytosolic Ca^"^ and diacylglycerol as second messengers. In many Systems, the effects of second messengers appear to be mediated by the activation of spécifie protein kinases that phosphorylate a variety of substrate proteins. Studies of protein kinases have already been performed in extracts of BAEC where cAMPdependent kinase, calmodulin (CaM) dependent protein kinase (CaM kinase II, CaM kinase III) and protein kinase C activities were detected (25); in addition, a kinase activity distinct from those mentioned above was measured in membranes of proliferating BAEC (26). However, except for a few preliminary (27, 28) or partial (29) studies, the patterns of protein phosphorylation in intact endothelial cells have not yet been fully characterized. In this paper, we show that ATP and bradykinin induce or enhance the phos phorylation of several proteins in intact BAEC, mostly via Ca^*dependent kinases. 18459