Coherent control of light shifts in an atomic medium driven by two orthogonally polarized pulses: Effect of the pulse overlap J. C. Delagnes and M. A. Bouchene Laboratoire de Collisions Agrégats Réactivité, C.N.R.S. UMR 5589, IRSAMC, Université Paul Sabatier, 118 Route de Narbonne, 31062 Toulouse Cedex 4, France Received 13 June 2007; published 8 November 2007 We consider a duplicated two-level system where each two-level subsystem is driven by a strong resonant femtosecond pulse and a weak resonant femtosecond pulse connects cross transitions. Strong interference effects are induced in such a configuration leading to a modulation of the medium gain as a function of the relative phase between the pulses J. C. Delagnes and M. A. Bouchene, Phys. Rev. Lett. 98, 053602 2007. We study here the influence of the temporal overlap between the pulses on the dynamics of the system and the medium gain. We show that the dynamics is dominated by two competing phenomena: Light shifts LS induced by the driving pulse that prevails for small delays and free induction decay FIDthat prevails for large delays. LS enhance the medium gain for = /2 and reduce it for =0, whereas FID always leads to a decrease of the medium gain. DOI: 10.1103/PhysRevA.76.053809 PACS numbers: 42.50.Gy, 42.50.Hz, 42.50.Md I. INTRODUCTION A lot of proposed methods to control physical and chemi- cal processes rely on the interference effects produced by excitation with coherent fields. The control is performed by adjusting the relative phase between the exciting fields which steers the interference of the quantum paths involved in the process. Such control has been demonstrated in many con- texts 1. An interesting scenario is the possibility to control physical processes or pulse wave form when propagation ef- fects are taken into account. Many previous studies have shown the dramatic modifications that occur in the behavior of the propagating pulses when the relative phase is modified 28. If strong pulses are used, light shifts LSare induced in the medium and strong modification occurs in the atomic structure. LS are the basis for many spectacular phenomena in atomic and molecular physics. Rapid adiabatic passage, stimulated Raman adiabatic passage, Stark-chirped adiabatic passage 9and light induced potential 10are nonexhaus- tive examples of effects where LS play a crucial role. The possibility to control these effects has been demonstrated in only few cases. One can use shaped intense femtosecond pulses to realize a selective population of dressed states 11. In a recent paper, we have demonstrated coherent control of LS effects in a duplicated two-level system 2. A sequence of two femtosecond coherent pulses—polarized strong pulse and polarized weak pulse—excite resonantly the S 1/2 - P 1/2 transition of atomic rubidium in an optically dense sample. The pulse induces transitions between the adia- batic states with a coupling that is different for either identi- cally or oppositely light-shifted states, and that can be modi- fied by tuning the relative phase between the pulses. An efficient control of the medium gain for the pulse was experimentally demonstrated. It was shown to be the result of the interference between the absorption and the emission quantum paths for photons. In that experiment, the delay between the two pulses was smaller than the pulse durations so the pulse overlap was almost perfect. In this paper, we study the influence of the pulse overlap on the medium gain and the LS effects. Spectacular changes occur with respect to the previous situation of perfect overlap. Indeed, the modifi- cation of the driving pulse area due to FID can no longer be neglected and LS effects are reduced. The competition be- tween FID and LS leads to a significant modification of the medium gain. The situation =0 for which destructive inter- ference occurs at zero delay may be more favorable for am- plification than the situation = / 2 that was the previous favorable case. II. COHERENT CONTROL OF LIGHT SHIFTS We consider the situation of a duplicated two-level system |1, |1', |2, |2' Fig. 1aexcited resonantly by two time delayed pulses. Pulse 1strongly couples the par- allel states while pulse 2which is weak couples resonantly the crossed states. In practice, this situation can be realized by exciting the atomic rubidium with a pair of - and -polarized pulses acting on the S 1/2 P 1/2 transition. The |2' > |1' > P 1/2 S 1/2 -1/2 +1/2 |1 > |2 > M J π π σ a) b) c) -iχ 2 sin φ iχ 2 sin φ -χ 2 cos φ |- > |+ > |-' > |+' > |2' > |1' > |1 > |2' > |2 > |1' > + |1 > |2 > π π π π σ + σ - e +iφ e -iφ d) z y x parallel parallel antiparallel prop. axis strong π pulse weak σ pulse FIG. 1. aEnergy levels and optical transitions involved in our system. bAdiabatic representation. cPolarization configuration. dAbsorption and emission paths. PHYSICAL REVIEW A 76, 053809 2007 1050-2947/2007/765/0538096©2007 The American Physical Society 053809-1