مح ی ط ز ی ست و مهندس ی آب
Environment and Water Engineering
دوره9 ، شماره2 ، ابستان ت1402
Vol. 9, No. 2, 2023
DOI: 10.22034/EWE.2022.350118.1798 Environ. Water Eng., 2023, 9(2), 179-194
ISSN: 2476-3683
Environment and Water Engineering
Homepage: www.jewe.ir
Research Paper
Liquid-Liquid Extraction of Penicillin-G from Pharmaceutical
Wastewater Via a Developed Polysulfone Hollow Fiber Membrane
Contactor
1
PhD Scholar, Department of Chemical Engineering, Gachsaran Branch, Islamic Azad University,
Gachsaran, Iran
2
Assist. Professor, Department of Chemical Engineering, Membrane Science and Technology
Research Center (MSTRC), Gachsaran Branch, Islamic Azad University, Gachsaran, Iran
3
Assist. Professor, Department of Chemical Engineering, Shiraz Branch, Islamic Azad University,
Shiraz, Iran
Article information Abstract
Received: July 24, 2022
Revised: September 01, 2022
Accepted: September 03, 2022
The presence of pharmaceutical wastewater can pose significant challenges
to the environment. Since conventional wastewater treatment processes are
not efficient for the complete separation of drug materials, solvent
extraction through a hollow fiber membrane contactor could be a promising
alternative. In this study, a developed polysulfone (PSF) hollow fiber
membrane was fabricated using a non-solvent phase separation (NIPS)
method to extract penicillin G from aqueous solutions in the membrane
contactor system. From the characterization experiments, the prepared
polysulfone membrane demonstrates an outer surface contact angle of
69.6°, critical water entry pressure (CEPw) of 250 kPa, total porosity of
72.2%, and collapsing pressure of 500 kPa. The extraction of penicillin G
from the aqueous phase was performed with a 5% w/w solution of Aliquat
336. The effect of the operating parameters on the extraction flux of
penicillin G was investigated using the response surface method (RSM).
The optimum penicillin G flux of 1.46×10
-3
kg/m
2
s was found at an
operating pressure of 100 kPa, an aqueous phase flowrate of 70.5 ml/min,
and an organic phase flowrate of 200 ml/min. Therefore, the developed PSF
hollow fiber membrane contactor can be considered a proper choice to
remove antibiotics (penicillin G) from aqueous solutions.
Keywords:
Fiber Membrane Contactor
Polysulfone
Antibiotic Extraction
Wastewater Treatment
*Corresponding author:
amir.mansourizadeh@iau.ac.ir
© Authors, Published by Environment and Water Engineering journal. This is an open-access
article distributed under the CC BY (license http://creativecommons.org/licenses/by/4.0/).
Introduction
The volume of antibiotics as causal pollutants in
the environment, especially aquatic
environments, has increased significantly. To
remove and recycle pollutants from hospitals and
urban and industrial wastewaters, membrane
technology has been designed. Membrane
contactor technology has been applied for gas
and liquid separation thanks to the advantages
such as high contact area, low operating pressure,
and high efficiency. Several studies on
Farzaneh Abbasi-Sourki
1
, Amir Mansourizadeh
2*
and Mohammad
Hossein Jazebizadeh
3