Citation: Arkas, M.; Bompotis, T.;
Giannakopoulos, K.; Favvas, E.P.;
Arvanitopoulou, M.; Arvanitopoulos,
K.; Arvanitopoulos, L.; Kythreoti, G.;
Vardavoulias, M.; Giannakoudakis,
D.A.; et al. Hybrid Silica Xerogel and
Titania/Silica Xerogel Dispersions
Reinforcing Hydrophilicity and
Antimicrobial Resistance of Leathers.
Gels 2023, 9, 685. https://doi.org/
10.3390/gels9090685
Academic Editors: Francesco Caridi,
Giuseppe Paladini and Andrea
Fiorati
Received: 23 July 2023
Revised: 19 August 2023
Accepted: 21 August 2023
Published: 25 August 2023
Copyright: © 2023 by the authors.
Licensee MDPI, Basel, Switzerland.
This article is an open access article
distributed under the terms and
conditions of the Creative Commons
Attribution (CC BY) license (https://
creativecommons.org/licenses/by/
4.0/).
gels
Article
Hybrid Silica Xerogel and Titania/Silica Xerogel Dispersions
Reinforcing Hydrophilicity and Antimicrobial Resistance
of Leathers
Michael Arkas
1,
* , Theofanis Bompotis
1
, Konstantinos Giannakopoulos
1
, Evangelos P. Favvas
1
,
Marina Arvanitopoulou
1
, Konstantinos Arvanitopoulos
2
, Labros Arvanitopoulos
2
, Georgia Kythreoti
3,4
,
Michail Vardavoulias
5
, Dimitrios A. Giannakoudakis
6
, Laura Castellsagués
7
and Sara Maria Soto González
7,8
1
Institute of Nanoscience Nanotechnology, NCSR “Demokritos”, Patriarchou Gregoriou Street,
15310 Athens, Greece; fanisbobotis@gmail.com (T.B.); k.giannakopoulos@inn.demokritos.gr (K.G.);
e.favvas@inn.demokritos.gr (E.P.F.); marinaarva3@gmail.com (M.A.)
2
DARVICHEM Alexandrou, Papagou 5, 18233 Agios Ioannis Rentis, Greece; darvichem@hol.gr (K.A.);
info@darvichem.gr (L.A.)
3
Institute of Bioscience and Applications, NCSR “Demokritos”, Patriarchou Gregoriou Street,
15310 Athens, Greece; gkythreoti@acg.edu
4
Department of Science and Mathematics, School of Liberal Arts and Sciences, The American College of
Greece, Deree, Gravias 6, 15342 Athens, Greece
5
PYROGENESIS S.A., Technological Park 1, Athinon Avenue, 19500 Attica, Greece;
mvardavoulias@pyrogenesis-sa.gr
6
Department Chemistry, Aristotle University of Thessaloniki, 54124 Thessaloniki, Greece; dagchem@gmail.com
7
Barcelona Institute for Global Health (ISGlobal), Universitat de Barcelona, 08036 Barcelona, Spain;
laura.castellsagues@isglobal.org (L.C.); sara.soto@isglobal.org (S.M.S.G.)
8
CIBER Enfermedades Infecciosas (CIBERINFEC), Instituto de Salud Carlos III, 28029 Madrid, Spain
* Correspondence: m.arkas@inn.demokritos.gr; Tel.: +30-210-6503669
Abstract: Four leather substrates from different animals were treated by dispersions containing
hydrophilic composite silica-hyperbranched poly(ethylene imine) xerogels. Antimicrobial activity
was introduced by incorporating silver nanoparticles and/or benzalkonium chloride. The gel pre-
cursor solutions were also infused before gelation to titanium oxide powders typically employed
for induction of self-cleaning properties. The dispersions from these biomimetically premade xe-
rogels integrate environmentally friendly materials with short coating times. Scanning electron
microscopy (SEM) provided information on the powder distribution onto the leathers. Substrate
and coating composition were estimated by infrared spectroscopy (IR) and energy-dispersive X-ray
spectroscopy (EDS). Surface hydrophilicity and water permeability were assessed by water-contact
angle experiments. The diffusion of the leather’s initial components and xerogel additives into
the water were measured by Ultraviolet-Visible (UV-Vis) spectroscopy. Protection against GRAM-
bacteria was tested for Escherichia coli, Pseudomonas aeruginosa, and Klebsiella Pneumoniae against
GRAM+ bacteria for Staphylococcus aureus and Enterococcus faecalis and against fungi for Candida
albicans. Antibiofilm capacity experiments were performed against Staphylococcus aureus, Klebsiella
Pneumoniae, Enterococcus faecalis, and Candida albicans. The application of xerogel dispersions proved
an adequate and economically feasible alternative to the direct gel formation into the substrate’s
pores for the preparation of leathers intended for medical uses.
Keywords: titanium oxide; antibacterial; antifungal; antibiofilm; hyperbranched; dendrimers;
polyethylene imine; IR spectroscopy; contact angle; electron dispersion spectroscopy
1. Introduction
The hides of killed animals were the obvious and abundant raw material used by
humanoids for protection against cold and other adverse environmental challenges. As
Gels 2023, 9, 685. https://doi.org/10.3390/gels9090685 https://www.mdpi.com/journal/gels