VOL. 2, NO. 3, April 2012 ISSN 2225-7217
ARPN Journal of Science and Technology
©2011-2012. All rights reserved.
http://www.ejournalofscience.org
170
Effect of Nano-Silica on Alkali Activated Water-Cooled Slag Geopolymer
1
H.M.Khater,
2
B.A.El-Sabbagh,
3
M.Fanny,
4
M.Ezzat,
5
M.Lottfy
Housing and Building National Research Centre (HBNRC)
87 El-Tahrir St., Dokki, Giza, P.O. Box 1770 Cairo
1
Email: Hkhater4@yahoo.com
ABSTRACT
Ground granulated blast furnace slag is a finely ground, rapidly chilled aluminosilicate melt material separated from
molten iron in the blast furnace as a by-product. Rapid cooling results in an amorphous or a glassy phase known as GGBFS
or water-cooled slag (WCS). Alkaline activation of latent hydraulic WCS by 6% sodium hydroxide was studied. Nano
silica is an ultrafine material that can modify mechanical, microstructural and thermal properties of geopolymer products
and added to the geopolymer mix in the ratio of 0, 0.50,1 and 1.5% of the dry weight. Curing was performed under 100%
relative humidity and at a temperature of 38
o
Keywords: Nano- silica, Geopolymer, Slag, Microstructure, Thermal properties.
C. Gelenium Ace super-plasticizer was added in the ratio of 4% from the dry
weight to ensure best dispersion of the nano silica. The results showed that increasing in the percentage of nano silica
results in enhancement in the mechanical properties as compared to the control mix up to 90 days. The study of thermal
properties is taken place for the different ratios by experimental and mathematical evaluation. The study showed that the
thermal properties as well as thermal insulation property are improved with the increase of ratio of nano silica.
1. INTRODUCTION
Geopolymers are inorganic polymeric
materials, firstly developed by Joseph Davidovits in
1970s. Geopolymerization involves a chemical reaction
between alumino-silicate oxides and alkali metal silicate
solutions under highly alkaline conditions yielding
amorphous to semi-crystalline three-dimensional
polymeric structures, which consist of Si–O–Al bonds
[1], and gave a fresh insight into this class of inorganic
polymer.
Geopolymerization is being considered for
replacing traditional structural materials and offers a
possible solution to the immobilization of toxic and
radioactive wastes as well as the treatment of industrial
wastes to produce value added construction materials.
Therefore, there is an increasing need for multiple source
materials to be jointly geopolymerised to maximally
exploit the respective properties of the individual sources
regarding compressive strength, stability and durability
[2].
Geopolymer can be thought of as a new
generation binder as a substitute for the calcium silicate
hydrate which are essential components of Portland
cement. Ordinary Portland Cement (OPC) is the main
ingredient used in the production of concrete-the most
widely used construction material in the world. In the
past, concrete was simply a composite of OPC paste
with aggregates, however, modern-day concrete
incorporates other cementitious materials, which act as
partial replacements of OPC. The manufacturing of OPC
requires the burning of large quantities of fuel, and
decomposition of limestone. Both, burning of fuel and
decomposition of limestone, result in significant
emissions of carbon dioxide. For every ton of OPC
manufactured, nearly one ton of CO
2
is produced
depending on the production process adopted [3].
Cement plants are reported to emit up to 1.5 billion tons
of CO
2
into the atmosphere annually [4,5]. Hence,
environmental preservation has become a driving force
behind the search for new sustainable and
environmentally friendly composites to replace
conventional concrete produced from OPC.
In 1978, Davidovits [6] introduced the word
‘geopolymer’ to describe an alternative cementitious
material, which has ceramic-like properties. As opposed
to OPC, the manufacture of aluminosilicate-based
geopolymer does not consume high levels of energy, as
water cooled slag (WCS), known also as ground
granulated blast furnace slag, is already an industrial by-
product. This geopolymer technology has the potential to
reduce emissions by 80% [3] because high temperature
calcining is not required. It also exhibits ceramic-like
properties with superior resistance to fire at elevated
temperatures. Geopolymer can be produced by
combining a pozzolanic compound or aluminosilicate
source material with highly alkaline solutions [7].