Physlca A 154 (1989) 511-520
North-Holland, Amsterdam
CRITICAL POINTS CHARACTERIZATION USING PROBABILITY
DISTRIBUTIONS
II. PHASE TRANSITION OF LIQUID BINARY MIXTURES
J GUI~MEZ, S VELASCO and A CALVO HERNANDEZ
Departamento de Ffsma, Facultad de Clenctas, Umversldad de Salamanca, 37008 Salamanca,
Spare
Received 15 July 1988
A renormahzatlon-group-hke method, developed m a preceding paper, Js apphed to
characterize critical points in hquld binary mixtures The method ~s based on the behavior of
the probability distribution associated to these systems Two examples are developed In the
first case (T-independent energy lnterachon between unhke molecules), the isomorphism wah
the llqmd-gas phase transition is estabhshed In the second one (T-dependent energy
lnterachon between unhke molecules), the difference between simple and double critical
points appearing m closed-loop phase diagrams Is reported
1. Introduction
In a preceding paper (hereafter referred to as paper I) a renormahzatton-
group-hke method based on the use of probablhty distributions is applied to
characterize the critical point and the coexistence line for the hqutd-gas phase
transalon [1]
In another recent paper [2] we have obtained the probablhty distribution for
a binary hquld model from which different temperature vs composition phase
diagrams can be reported In particular, closed-loop phase-diagrams [3] with
upper (UCT) and lower (LCT) critical temperatures have been obtained
Furthermore, analytic calculations have been carried out by assuming an
explicit and simple T-dependence of the interaction energy between unhke
molecules In the case that the closed loop reduces to a point, upper and lower
crlttcal temperatures coincide and the critical point is a double critical point
The present work is devoted to apply the method developed m paper I to
hquld binary rnlxtures, in order to characterize the different critical points
(single, upper and lower, double) appearing in these systems
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