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American Journal of Essential Oils and Natural Products 2014; 2(1): 19-23
ISSN: 2321 9114
AJEONP 2014; 2(1): 19-23
© 2014 AkiNik Publications
Received: 03.07.2014
Accepted: 18.09.2014
Yahima Frión-Herrera
Food and Pharmacy Institute,
Havana University, Cuba
Alexis Díaz-García
Laboratories of Biopharmaceuticals
and Chemistry Productions
(LABIOFAM) Ave.
Independencia, Km 16 ½,
Stgo de las Vegas, Boyeros. La
Habana, Cuba
Hermis Rodríguez-Sánchez
Microbiology Department, Tropical
Medicine Institute “Pedro Kouri”
Havana, Cuba
Jenny L. Ruiz-Fuentes
Microbiology Department, Tropical
Medicine Institute “Pedro Kouri”
Havana, Cuba
Lianet Monzote Fidalgo
Microbiology Department, Tropical
Medicine Institute “Pedro Kouri”
Havana, Cuba
William N. Setzer
Department of Chemistry,
University of Alabama in
Huntsville, Huntsville, AL 35899,
USA
Correspondence:
Alexis Díaz-García
Laboratories of Biopharmaceuticals
and Chemistry Productions
(LABIOFAM) Ave.
Independencia, Km 16 ½,
Stgo de las Vegas, Boyeros. La
Habana, Cuba
Cytotoxic effect of Cuban propolis extracts on normal
cells and in-vitro basal toxicity assay to estimate acute
oral toxicity
Yahima Frión-Herrera, Alexis Díaz-García, Hermis Rodríguez-Sánchez,
Jenny L. Ruiz-Fuentes, Lianet Monzote Fidalgo and William N. Setzer
Abstract
In-vitro toxicity tests are recognized as alternative methods to animal acute toxicity testing. The aim of
this study was to assess toxicity of 16 Cuban propolis extracts of different chemical types: brown (1, 4, 5,
16, and 17 BCP), red (9, 29, 35, 37, 45 and 72 RCP) and yellow (18, 39, 41, 50 and 60 YCP) against
Balb/c 3T3 and Vero cells. Cells were treated at different concentrations (12.5; 25; 50 and 100 μg/mL) of
propolis for 72 h and the IC50 value was determined. Furthermore we employed in-vitro cytotoxicity test
described by Spielmann et al., red uptake (NRU) assay to estimate acute oral toxicity. Propolis showed
differential cytotoxicity toward normal cells in a dose and tissue-dependence. RCP was the most
interesting group because they did not affect normal cells evaluated. In Balb/c 3T3-A31 NRU
cytotoxicity assay, after incubation for 48 h, IC50 values to RCP-45 and RCP-37 were 86.8 ± 1.14 and
96.1 ± 1.02 µg/mL, respectively. The LD50 values of these extracts were 558 and 579 mg/kg,
respectively. For both samples the start dose for acute oral toxicity studies is 550 mg/kg in the case of
using the Up-and-Down Procedure (UDP) and 300 mg/kg when Fixed Dose Procedure (FDP) and Acute
Toxic Class Methods (ATC) were used. Results presented in this work can contribute to understand the
toxicological profile of Cuban propolis and reduce the number of animals required in subsequent
pharmacological / toxicological studies.
Keywords: Cuban propolis, cytotoxicity, normal Cells, NRU assay.
1. Introduction
Natural products constitute one of the most promising sources to obtain biologically active
compounds. During the last decade, propolis has been found to exhibit a broad spectrum of
therapeutic effects, including antibacterial, antifungal, antitumor, antioxidant,
immunomodulatory and other beneficial properties
[1, 2]
. This bee product is derived from
various plant resins and widely employed in traditional medicine.
Cuban propolis has been classified according to its composition: brown Cuban propolis type
(BCP type), rich in polyisoprenylated benzophenones
[3]
, red type (RCP type), containing
isoflavonoids as the main constituents, and yellow type (YCP type) with a variety of
triterpenoids as the major chemical components
[4]
. Recently, extracts of BCP, RCP and YCP
have shown potential activity against tumor cells, using murine breast carcinoma, human
breast adenocarcinoma and human lung adenocarcinoma
[5]
, and antiprotozoal properties
against Leishmania amazonensis, Trichomonas vaginalis and Plasmodium falciparum
[6,7]
. In
this sense, extensive cytotoxic studies should be carried out with Cuban propolis.
Therefore, is reasonable to use, at the primary screening stage, in-vitro toxicity assays on
normal cells to select the less toxic compounds among the most active ones. The toxicological
potential of a compound is analyzed through the affectation of vital functions of normal and
tumor cell lines from different tissues and different species
[8]
. Moreover, the fulfilling of this
criterion and also the combination with the estimation of the initial dose for acute toxicity tests
in rodents, using in-vitro data, facilitate the selection of the most promising compounds while
the reduction of laboratory animals is accomplished
[9]
.
Basal cytotoxicity is considered the starting point for an integrated assessment of potential in-
vivo acute systemic toxicity
[10, 11]
.