Hydrogen production methods efficiency coupled
to an advanced high-temperature accelerator
driven system
Daniel Gonz
alez Rodrı´guez
a,*
, Carlos Alberto Brayner de Oliveira Lira
b
,
Carlos Rafael Garcı´a Hern
andez
c
, Fernando Roberto de Andrade Lima
a
a
Centro Regional de Ci^ encias Nucleares Do Nordeste CRCN-NE, Avenida Professor Luiz Freire, 1000 50740-535
Recife, PE, Brazil
b
Departamento de Energı´a Nuclear, Universidade Federal de Pernambuco, Avenida Professor Luiz Freire, 1000
50740-535 Recife, Brazil
c
Instituto Superior de Tecnologı´as y Ciencias Aplicadas (InSTEC/CUBA), Av. Salvador Allende Esq, Luaces 10400 La
Habana, Cuba
article info
Article history:
Received 26 July 2018
Received in revised form
31 October 2018
Accepted 11 November 2018
Available online xxx
Keywords:
Nuclear hydrogen production
ADS
HTE
Sulfur-iodine
Efficiency
Cost estimative
abstract
Hydrogen, rather than oil, must be produced in volumes not provided by the currently
employed methods. In this work, two high-temperature hydrogen production methods
coupled with an advanced nuclear system are presented. A new design of a pebble-bed
accelerator nuclear-driven system called TADSEA (Transmutation Advanced Device for
Sustainable Energy Applications) was chosen because of the advantages in transmutation
and safety. A detailed flowsheet of the high-temperature electrolysis process coupled to
TADSEA through a Brayton gas cycle was developed using chemical process simulation
software: Aspen HYSYS
®
. It is obtained 0.1627 kg/s of hydrogen with the model with
optimized operating conditions, resulting in an overall process efficiency of 34.51%, a value
in the range of results reported by other authors. A conceptual design of a plant using the
iodine-sulfur thermochemical water splitting cycle was carried out producing 5.66e-2 kg/s
and electric energy in cogeneration. The overall efficiency was calculated performing an
energy balance resulting in 22.56%. A brief hydrogen production cost estimation was per-
formed for both methods obtaining 5.96$/kg for the sulfur-iodine (SI) and 4.8 $/kg for the
high-temperature electrolysis (HTE) process.
© 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Introduction
Hydrogen is considered as the basis of the near future energy
system. The progressive replacement of oil can help reduce
the environmental impacts associated with the production
and use of it. Hydrogen combustion does not produce green-
house gases, but the application of hydrogen in the future will
be as an energy carrier rather than fuel [1]. An energy carrier is
a substance that can store energy so that it can be later
consumed in a controlled manner. The energy carriers differ
from the primary energy sources because they need to be
* Corresponding author.
E-mail addresses: danielgonro@gmail.com (D. Gonz alez Rodrı´guez), cabol@ufpe.br (C.A. Brayner de Oliveira Lira), cgh@instec.cu
(C.R. Garcı´a Hern andez).
Available online at www.sciencedirect.com
ScienceDirect
journal homepage: www.elsevier.com/locate/he
international journal of hydrogen energy xxx (xxxx) xxx
https://doi.org/10.1016/j.ijhydene.2018.11.083
0360-3199/© 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Please cite this article as: Gonz alez Rodrı´guez D et al., Hydrogen production methods efficiency coupled to an advanced high-tem-
perature accelerator driven system, International Journal of Hydrogen Energy, https://doi.org/10.1016/j.ijhydene.2018.11.083