Available online at www.sciencedirect.com
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Materials Today: Proceedings 5 (2018) 23586–23595 www.materialstoday.com/proceedings
2214-7853© 2018 Elsevier Ltd. All rights reserved.
Selection and/or Peer-review under responsibility of International Conference on Advances in Materials and Manufacturing Applications
[IConAMMA 2017].
IConAMMA_2017
Cure and Degradation Kinetics of Sulfur Cured Nanocomposites of
EPDM-NBR Rubber Blends
Sanha Kaizer Tajamul Basha
a
, Divya R
a
, Ashwini U Menon
a
, Neelesh Ashok
a,b
,
Meera Balachandran
a,b*
a
Department of Chemical Engineering and Materials Science, Amrita School of Engineering, Coimbatore, Amrita Vishwa Vidyapeetham, Amrita
University, India
b
Centre of Excellence in Advanced Materials and Green Technologies(CoE-AMGT), Amrita School of Engineering, Coimbatore, Amrita Vishwa
Vidyapeetham, Amrita University, India
Abstract
Ethylene Propylene Diene Monomer (EPDM) rubber is widely used in nuclear plants due to its resistance to radiation, which is
highest among elastomers. However, owing to its poor resistance to aliphatic hydrocarbons, components made of EPDM fail
when exposed to environments that have the combined effect of radiation and hydrocarbons. The life of such components can be
extended by blending EPDM with a hydrocarbon resistant polymer like nitrile rubber (NBR). By incorporating nanoparticles like
nanoclay in the rubber blend, properties like hydrocarbon resistance, radiation resistance and mechanical properties can be
improved. In this work, detailed analysis of cure characteristics, cure kinetics and degradation kinetics of EPDM - NBR blend
based nanocomposites with nanoclay as filler is presented. Kinetic analysis gives a detailed insight into the mechanisms of the
reactions of curing and degradation which affects the characteristics of the final product. The miscibility of EPDM – NBR blends
with maleic anhydride as compatibilizer was ascertained by Differential Scanning Calorimetry. The cure and degradation kinetics
of the nanocomposites were analysed as a function of nanoclay content. The order of the reaction was found to be one, for cure
and degradation reactions. Also, the rate constant of the cure and degradation reactions increased with concentration of
nanoclayand then declined with increase in nanoclay content.The observed results were correlated to the morphology of
nanocomposites.
© 2018 Elsevier Ltd. All rights reserved.
Selection and/or Peer-review under responsibility of International Conference on Advances in Materials and Manufacturing Applications
[IConAMMA 2017].
Keywords:curing; degradation; kinetics; rubber; nanocomposites.
* Corresponding author. Tel.: +91(422) 2685000; fax: +91(422) 2656274.
E-mail address: b_meera@cb.amrita.edu