Jointly published by React.Kinet.Catal.Lett.
Akadémiai Kiadó, Budapest Vol. 90, No. 2, 381–387 (2007)
and Springer, Dordrecht 10.1007/s11144-007-4938-2
0133-1736/2007/US$ 20.00.
© Akadémiai Kiadó, Budapest.
All rights reserved.
RKCL4938
TEMPLATED SYNTHESIS AND CATALYTIC PROPERTIES OF AN
Rh/CERIA-ZIRCONIA CATALYST
Jin An Wang
a, *
, Gabliela González
1
, Lifang Chen
b
,
Miguel A. Valenzuela
b
, Maria Moran-Pineda
c
, Armando Vázquez
c
and Salvador Castillo
c
a
Laboratorio de Catálisis y Materiales, ESIQIE, Instituto Politécnico Nacional,
Col. Zacatenco, 07738 México D.F., México
b
Departamento de Ciencias Básicas, Universidad Autónoma Metropolitana-A, Av. San Pablo 180,
Col. Reynosa-Tamaulipas, 02200 México D.F., México
c
Instituto Mexicano del Petróleo, Programa de Ingeniería Molecular, Eje Central Lázaro Cárdenas
No. 152, 07730 México D. F, México
Received January 8, 2007, accepted January 22, 2007
Abstract
Ceria-zirconia nanophase with structural defects and high thermal stability was
synthesized by a surfactant-templated method. The 0.5 wt.% Rh/ceria-zirconia
catalyst shows high activity for NO reduction by CO under an oxygen-rich
condition, and the selectivity to 100% N
2
below 200°C was achieved.
Keywords: Ceria-zirconia, surfactant-templated synthesis, NO reduction
INTRODUCTION
Nowadays, ceria-zirconia mixed oxides have been widely applied as catalyst
support in the new generation of the automotive three-way catalyst (TWC)
converter due to their high oxygen storage capacity and redox property [1,2].
___________________________
* Corresponding author. Tel. (52) 55 57296000 ext. 55261; Fax. (52) 55 55862728
E-mail: wang_j_a@yahoo.com; jwang@ipn.mx