Int. J. Environment and Sustainable Development, Vol. 11, No. 1, 2012 3
Copyright © 2012 Inderscience Enterprises Ltd.
Mercury mobility and availability in highly
contaminated solid wastes from a chlor-alkali plant
Yailen Busto*
Study Center of Applied Chemistry,
Faculty of Chemistry and Pharmacy,
Central University “Marta Abreu” of Las Villas,
Camajuani Road, Km 5 1/2,
54830, Santa Clara, Villa Clara, Cuba
E-mail: BustoYera.Yailen@ugent.be
E-mail: yailenb@uclv.edu.cu
*Corresponding author
Filip Tack
Department of Applied Analytical and Physical Chemistry,
Ghent University,
Coupure Links 653,
B-9000 Ghent, Belgium
E-mail: filip.tack@ugent.be
Xiomara Cabrera
Chemical Engineering Department,
Faculty of Chemistry and Pharmacy,
Central University “Marta Abreu” of Las Villas,
Camajuani Road, Km. 5 1/2,
54830, Santa Clara, Villa Clara, Cuba
E-mail: qfx@uclv.edu.cu
Abstract: This article suggests an approach of sustainable development in
Cuba based on the environmental impact assessment of mercurial sludge
generated by a chlor-alkali Cuban plant. It consists of a study of mercury
mobility and availability in the sludge samples using sequential extraction
procedure. High values of total mercury content (2320 ± 40 mg/kg) in the
sludge sample as well as in the toxicity characteristic leaching procedure
(TCLP) extract (0.46 ± 0.02 mg/l) were obtained. The highest Hg concentration
(52.2 ± 1.5%) was found in the mobile fraction (F1 + F2) indicating a high risk
of Hg mobilisation by the presence of water-soluble and exchangeable mercury
compounds such as HgCl
2
, HgSO
4
and HgO. The water-soluble fraction (F1)
accounts for the 13.7 ± 0.8% of total Hg representing a significant
environmental risk due to its easy availability in environmental weathering
conditions. The mercury fractionation analyses clearly demonstrate that the
chlor-alkali Cuban plant does not represent a sustainable technology from
environmental point of view. Furthermore, this study highlights the presence of
a wide range of mercury compounds which represents a significant parameter
for developing a sustainable technology to treat the mercurial sludge generated
by the chlor-alkali Cuban plant.