European Reviews of Chemical Research, 2015, Vol.(6), Is. 4
Copyright © 2015 by Academic Publishing House Researcher
Published in the Russian Federation
European Reviews of Chemical Research
Has been issued since 2014.
ISSN: 2312-7708
E-ISSN: 2413-7243
Vol. 6, Is. 4, pp. 192-211, 2015
DOI: 10.13187/ ercr.2015.6.192
www.ejournal14.com
UDC 541.64:574.24:553.08
The Methods of non-equilibrium Spectrum (NES) and Differential non-equilibrium
Spectrum (DNES) in Studying the Interaction of Carbonaceous Mineral Shungite
and Aluminosilicate Mineral Zeolite with Water
1
Ignat Ignatov
2
Oleg Mosin
1
Th e Scientific Research Center of Medical Biophysics (SRC MB), Bulgaria
Professor, D. Sc., director of SRC MB
1111, Sofia, N. Kopernik street, 32
E-mail: mbioph@dir.bg
2
Moscow State University of Applied Biotechnology, Russian Federation
Senior research Fellow of Biotechnology Department, Ph. D. (Chemistry)
103316, Moscow, Talalihina ulitza, 33
E-mail: mosin-oleg@yandex.ru
Abstract
The mathematical model of interaction with water the amorphous, uncrystallized, fullerene
analogous carbon containing natural mineral shungite (Zazhoginskoe deposit, Karelia, Russia) and
micro-porous alumosilicate mineral zeolite (Most, Bulgaria) was established. There are submitted
data on the nanostructure and structural properties of these minerals, obtained with using the
elemental analysis, transmission electron microscopy (TEM-method) and IR-spectroscopy.
For evaluation of the mathematical model of interaction of these minerals with water, the methods
of non-equilibrium spectrum (NES) and differential non-equilibrium spectrum (DNES) of water
were applied. The values of average energy (∆EH...O
) of hydrogen Н…O-bonds among H
2
O
molecules in water samples after the treatment of shungite and zeolite with water was measured at
-0,1137 eV for shungite and -0,1174 eV for zeolite. The calculation of ∆E
H...O
for shungite with using
the DNES method compiles +0,0025±0,0011 eV and for zeolite -1,2±0,0011 eV. It was
demonstrated a regularity of change of energy of hydrogen bonds between H
2
O molecules in the
process of water treatment by shungite and zeolite with a statistically reliable increase of local
maximums in DNES-spectra.
Keywords: shungite, zeolite, nanostructure, fullerens, IR, NES, DNES
Introduction
Shungite and zeolite – the minerals refer to new generation of natural mineral sorbents
(NMS). Shungite is an intermediate form between the amorphous carbon and the graphite crystal,
containing carbon (30 %), silica (45 %), and silicate mica (about 20 %) [1]. The schungite carbon is
a fossilized organic material of the sea bottom Precambrian sediments of high level of
carbonization containing the fullerene-like regular structures. Shungite got its name after the
village of Shunga in Karelia (Russian Federation), located on the shore of Onezhskoe Lake, where is
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