Materials Sciences and Applications, 2018, 9, 844-857
http://www.scirp.org/journal/msa
ISSN Online: 2153-1188
ISSN Print: 2153-117X
DOI: 10.4236/msa.2018.910061 Sep. 29, 2018 844 Materials Sciences and Applications
Synthesis and Characterization of Metal
Organic Chemical Vapour Deposited Chromium
Doped Zinc Oxide Thin Film for Gas Sensing
Applications
Olumide Oluwole Akinwunmi
1*
, Olakunle A. Akinwumi
1
, Johnson Ayodele O. Ogundeji
1
,
Adetokunbo Temitope Famojuro
2
1
Department of Physics and Engineering Physics, Obafemi Awolowo University, Ile-Ife, Nigeria
2
Department of Chemistry, Obafemi Awolowo University, Ile-Ife, Nigeria
Abstract
Chromium (Cr) doped Zinc oxide ZnO thin films were deposited onto glass
substrates by Metal Organic Chemical Vapour Deposition (MOCVD) tech-
nique with varying dopant concentration at a temperature of 420˚C. The effect
of the chromium concentration on morphological, structural, optical, electrical
and gas sensing properties of the films were investigated. The scanning elec-
tron microscopy results revealed that the Cr concentration has great influence
on the crystallinity, surface smoothness and grain size. X-ray diffraction
(XRD) studies shows that films were polycrystalline in nature and grown as
a hexagonal wurtzite structure. A direct optical band energy gap of 3.32 to
3.10 eV was obtained from the optical measurements. The transmission was
found to decrease with increasing Cr doping concentration. Rutherford Back-
scattering Spectroscopy (RBS) analysis also demonstrates that Cr ions are
substitutionally incorporated into ZnO. I-V characteristic of the film shows a
resistivity ranges from 1.134 × 10
-2
Ω cm to 1.24 × 10
-2
Ω cm at room temper-
ature. The gas sensing response of the films were enhanced with incorporation
of Cr as a dopant with optimum operating temperature around 200˚C.
Keywords
Zinc Oxide, Thin Films, Metal Organic Chemical Vapour Deposition,
Gas Sensors
1. Introduction
ZnO has been found invaluable in the development of new technologies based
How to cite this paper: Akinwunmi, O.O.,
Akinwumi, O.A., Ogundeji, J.A.O. and
Famojuro, A.T. (2018) Synthesis and Cha-
racterization of Metal Organic Chemical
Vapour Deposited Chromium Doped Zinc
Oxide Thin Film for Gas Sensing Applica-
tions. Materials Sciences and Applications,
9, 844-857.
https://doi.org/10.4236/msa.2018.910061
Received: August 30, 2018
Accepted: September 26, 2018
Published: September 29, 2018
Copyright © 2018 by authors and
Scientific Research Publishing Inc.
This work is licensed under the Creative
Commons Attribution International
License (CC BY 4.0).
http://creativecommons.org/licenses/by/4.0/
Open Access