American Journal of Chemistry 2015, 5(3A): 1-6
DOI: 10.5923/c.chemistry.201501.01
Extraction of Cd(II) Ions by Emulsion Liquid Membrane
(ELM) Using Aliquat 336 as Carrier
A. L. Ahmad
1,*
, M. M. H. Shah Buddin
1,2
, B. S. Ooi
1
1
School of Chemical Engineering, Universiti Sains Malaysia, Engineering Campus, Nibong Tebal, Malaysia
2
Fakulti Kejuruteraan Kimia, Universiti Teknologi MARA, Shah Alam, Malaysia
Abstract In this work, the potentialities of vegetable oil to be incorporated as diluent in Emulsion Liquid Membrane
(ELM) formulation was explored. Vegetable oil tested in this study are sunflower, corn and palm oil. A compatibility study
was conducted to investigate its feasibility to be used as diluent in ELM. It is learned that corn oil showed a promising results
to be incorporated in ELM to dissolve Span 80 and Aliquat 336 as surfactant and carrier in the membrane phase, respectively.
The analysis showed that Aliquat 336 is highly selective towards Cd(II) as it able to remove almost all Cd(II) ions from the
aqueous solution while Span 80 has assisted in the formation of a stable emulsion. The W/O emulsion was prepared using
0.1M NaOH as the internal phase while the membrane phase consist of 3 wt% Span 80 and Aliquat 336, dissolved in corn oil.
The influence of stirring speed and extraction time on the solute removal efficiency was observed. The best performance of
ELM in extracting Cd(II) ions was recorded at speed of 300 rpm for 15 min. 98.6% of Cd(II) ions were successfully removed
from the external aqueous phase at this condition.
Keywords Emulsion Liquid Membrane, Aliquat 336, Vegetable oil diluent, Cd(II) ions Extraction
1. Introduction
Rapid industrialization which begun in 1960s has raised
many critical issues regarding environmental pollution. One
of them is the emission of heavy metal with a great
potential to pollute the environment. In fact, Elbagermi et al.
[1] reported on the dramatic increasing trend of heavy metal
emission since the onset of industrial revolution. In the year
2013 alone, Department of Environment Malaysia reported
that a total of 103,994.37 metric tonnes of industrial waste
containing heavy metals were generated from various
industries in this country [2]. Among the most common
heavy metal found in polluted water includes arsenic,
copper, cadmium, lead, chromium, nickel, mercury and zinc
[3]. Apart from its ability to harm the ecosystem, extensive
study carried out by World Health Organization (WHO) has
revealed that exposure to these metals will eventually cause
deleterious health effects in humans though some of them
are nutritionally essential for a healthy life, but in a very
small quantity [4].
As for cadmium, it is a toxic metal occurring naturally in
the environment and it is considered as a pollutant emanating
primarily from industrial and agricultural sources [5]. Due to
its high solubility, cadmium can be easily absorbed by living
* Corresponding author:
chlatif@usm.my (A. L. Ahmad)
Published online at http://journal.sapub.org/chemistry
Copyright © 2015 Scientific & Academic Publishing. All Rights Reserved
organisms and it can easily enters our food chain [6]. Study
conducted by Kadaruddin [7] discovered that as much as 53
rivers in Malaysia’s river system were badly contaminated
with cadmium from various sources, mainly manufacturing.
Tremendous efforts have been carried out in minimizing
the concentration of heavy metal in aqueous media using
various physico-chemical treatment [8]. However, Emulsion
Liquid Membrane (ELM) which was invented by Li [9] has
shown a promising potential in the field of separation. In
case of metal removal from aqueous media, ELM was
reported to be successfully used in extracting numerous
types of heavy metal ions for instance, Cr(VI) [10], Cu(II)
[11] and Co(II) [12]. In addition, our previous work on ELM
using TOA as carrier has recorded more than 98% of
efficiency [13]. In this study, Aliquat 336 was used as the
carrier to specifically extract Cd(II) ions. Aliquat 336 is a
quaternary ammonium salts which reported to act as anion
exchanger at wide range of feed pH [14] and its viscous
characteristic has allowed the formation of a stable emulsion
against shear. In fact, Aliquat 336 possess surfactant
property [15] which is favourable in the production of a
stable emulsion.
ELM is a developed form of solvent extraction, with the
difference that extraction and stripping process occur
synchronously in the same unit [16]. In principal, ELM
consists of internal (W) and external (W) phase and they
were separated by the immiscible organic membrane phase
(O) thus, forming W/O/W (water-in-oil-in-water) emulsion
system. In this multiple emulsion system, the primary W/O