ISSN 0030-400X, Optics and Spectroscopy, 2014, Vol. 116, No. 3, pp. 379–383. © Pleiades Publishing, Ltd., 2014.
Original Russian Text © A.S. Shcheulin, A.E. Angervaks, A.V. Veniaminov, V.V. Zakharov, A.I. Ryskin, 2014, published in Optika i Spektroskopiya, 2014, Vol. 116, No. 3, pp. 408–
412.
379
Recording of holograms in ionic crystals with color
centers occurs according to the diffusion-drift mecha-
nism, according to which the centers undergo trans-
formation from one type into another and spatial
redistribution [1, 2]. The essence of this mechanism is
as follows: the radiation that is used to record a holo-
gram causes photoionization of color centers, which
are associates of anionic vacancies and electrons; their
number is the same as in the neutral state. This num-
ber varies from unity (F centers) to several tens and
even hundreds of thousands (highly aggregated cen-
ters). The electrons formed under these conditions
diffuse from maxima of the interference field to its
minima and are captured by traps (i.e., color centers)
[3]. As a result, an electric field is induced between the
maxima and minima. Anionic vacancies, being split
from an ionized center due to the thermal effect (holo-
grams are recorded in these crystals at a rather high
temperature) or formed due to its ionization (if the
case in point is an F center), drift under the field
toward interference minima. Here, they recombine
with the electrons released as a result of thermal ion-
ization of traps and form color centers. Thus, color
centers move from maxima to minima of the interfer-
ence field in which a hologram is recorded, although
the real motion is performed by their components.
This process can be accompanied by a change in the
center type, because the conditions under which color
centers are formed in minima differ from the condi-
tions corresponding to the formation of the “initial”
(i.e., photoionized in maxima) centers.
The diffusion-drift mechanism of hologram
recording proposed for alkali-halide crystals with
color centers in [1, 2] was used to describe the record-
ing of holograms on color centers in CaF
2
(fluorite)
crystals in [4]. In this paper, we report the results of
studying the mechanisms of transformation of color
centers during hologram recording in CaF
2
crystals.
To form color centers in a CaF
2
crystal, the latter
was subjected to additive coloring (heating in cation
metal vapor [5–7]). As a result, anionic vacancies and
electrons with a concentration of ~10
17
cm
–3
were
introduced into the crystal. “Simple” color centers (F,
M, R, and N) are generally formed at this (relatively
low) concentration. They are composed of one to four
anionic vacancies, respectively, with the same num-
bers of electrons and a small number of the so-called
“colloidal” centers, which are highly aggregated; these
are two-dimensional calcium inclusions in the fluorite
lattice [8, 9]. A plate 10 × 10 × 1.2 mm in size was cut
from a colored crystal. Its absorption spectrum, mea-
sured with a Cary 500 spectrophotometer, is shown in
Fig. 1. Colloidal centers manifest themselves in the
form of a weak shoulder near ~600 nm; other absorp-
tion bands are due to simple centers.
A hologram was recorded in the sample by 532-nm
radiation (a Cobolt Samba laser with an output power
of 500 mW) at a temperature of 190°С in a thermo-
stated interferometer, according to a symmetric trans-
mission scheme with a convergence angle of 2.7° on a
10 × 10-mm face; this angle value provided a holo-
graphic-grating period of 11 μm. The contrast of a
sinusoidal interference field recorded in the form of a
hologram was no less than 99%. The exposure during
recording was 31 kJ/cm
2
.
The absorption spectrum of the sample with a
recorded hologram is also shown in Fig. 1. One can see
that the recording leads to a significant increase in the
CONDENSED-MATTER
SPECTROSCOPY
Transformation of Color Centers during Hologram Recording
in an Additively Colored CaF
2
Crystal
A. S. Shcheulin, A. E. Angervaks, A. V. Veniaminov, V. V. Zakharov, and A. I. Ryskin
University ITMO, 197101 Russia
e-mail: angervax@mail.ru
Received September 17, 2013
Abstract—When holograms are recorded on color centers in calcium fluoride crystals, these centers undergo
spatial redistribution in the crystal bulk, which is accompanied by their transformation. The nature of this
transformation has been investigated by optical spectroscopy and confocal scanning microscopy. It is shown
that, under the recording conditions we used, the degree of center aggregation increases in both minima and
maxima of the interference field in which the recording performed. The enhanced aggregation in field min-
ima is caused by the increase in the concentration color centers, while the additional aggregation in maxima
is determined by the specific conditions of hologram recording: the wavelength and power density of record-
ing radiation and the crystal temperature.
DOI: 10.1134/S0030400X14030187