PHYSICAL REVIEW A 89, 053820 (2014)
High-average-power, 100-Hz-repetition-rate, tabletop soft-x-ray lasers at sub-15-nm wavelengths
Brendan A. Reagan,
1, 2, *
Mark Berrill,
1, 3
Keith A. Wernsing,
1, 2
Cory Baumgarten,
1, 4
Mark Woolston,
1, 2
and Jorge J. Rocca
1, 2, 4
1
NSF Engineering Research Center for Extreme Ultraviolet Science and Technology, Colorado State University,
Fort Collins, Colorado 80523, USA
2
Department of Electrical and Computer Engineering, Colorado State University, Fort Collins, Colorado 80523, USA
3
Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA
4
Department of Physics, Colorado State University, Fort Collins, Colorado 80523, USA
(Received 31 March 2014; published 15 May 2014)
Efficient excitation of dense plasma columns at 100-Hz repetition rate using a tailored pump pulse profile
produced a tabletop soft-x-ray laser average power of 0.1 mW at λ = 13.9 nm and 20 μW at λ = 11.9 nm from
transitions of Ni-like Ag and Ni-like Sn, respectively. Lasing on several other transitions with wavelengths between
10.9 and 14.7 nm was also obtained using 0.9-J pump pulses of 5-ps duration from a compact diode-pumped
chirped pulse amplification Yb:YAG laser. Hydrodynamic and atomic plasma simulations show that the pump
pulse profile, consisting of a nanosecond ramp followed by two peaks of picosecond duration, creates a plasma
with an increased density of Ni-like ions at the time of peak temperature that results in a larger gain coefficient
over a temporally and spatially enlarged space leading to a threefold increase in the soft-x-ray laser output pulse
energy. The high average power of these compact soft-x-ray lasers will enable applications requiring high photon
flux. These results open the path to milliwatt-average-power tabletop soft-x-ray lasers.
DOI: 10.1103/PhysRevA.89.053820 PACS number(s): 42.55.Vc, 52.38.Ph
I. INTRODUCTION
The great interest in sources of bright coherent soft-x-
ray radiation that has motivated the construction of free-
electron lasers [1,2] (FELs) also motivates the development
of more readily accessible tabletop soft-x-ray laser (SXRL)
sources. Despite the significant progress recently made in
both compact high-harmonic-generation-based sources [3,4]
and plasma-based SXRLs [5–15], their average power is at
present lower than that delivered by soft-x-ray FEL facilities
[1,2]. The average power of laser-pumped SXRLs has been
limited by the relatively low repetition rate of the high-energy
optical wavelength pump lasers used to drive them and
by low pumping efficiency. In contrast, capillary discharge
lasers are capable of milliwatt average power [16,17], but
currently their wavelengths are limited to values longer than
46 nm [18]. For laser-pumped soft-x-ray lasers operating
in the (10–15)-nm wavelength range, thermal effects within
the flash-lamp-pumped solid-state driver lasers have limited
the repetition rate to 10 Hz or less, resulting in maximum
average powers ranging from 1 to 20 μW[8,10]. Recently, we
reported a tabletop SXRL capable of 100-Hz-repetition-rate
operation, generating 0.15-mW average power on the λ =
18.9-nm line of Ni-like Mo [19], including the hour-long
operation of this laser at high repetition rates [20]. Here we
report the demonstration of a 0.1-mW-average-power, gain-
saturated, λ = 13.9-nm soft-x-ray laser operating at 100-Hz
repetition rate made possible by combining a high-energy
chirped pulse amplification (CPA) infrared laser pumped by
laser diodes that delivers pulses of up to 1 J of energy at this
repetition rate, with a temporally tailored infrared driver laser
pulse that more efficiently pumps the plasma amplifier.
The plasma amplifiers were excited by a single-shaped
pump pulse. Although the use of a single pulse has been
*
brendan.reagan@colostate.edu
used to drive tabletop soft-x-ray lasers before [9,13,19],
the pulse employed here has different characteristics. The
advantage of shaping the temporal sequence of pulses used
to efficiently create and heat soft-x-ray plasma amplifiers has
been recognized [7,13]. In particular it was shown that the
addition of a short-duration [2-ps full width at half maximum
(FWHM)] prepulse with a fraction of the intensity of the
main pulse can significantly increase the soft-x-ray laser pulse
energy produced by a λ = 13.9-nm Ni-like Ag laser when
pumping with relatively low driving laser pulse energies [7].
In another paper this work was expanded upon to allow the
generation of 4.7-μJ pulses at λ = 13.9 nm using less than 2 J
of total pump laser energy [21]. In recent previous work we
used a single tailored pump laser pulse to drive strong lasing in
the λ = 18.9-nm transition of Ni-like Mo at 100-Hz repetition
rate that resulted in an average power of 0.15 mW [19]. Here, in
order to more efficiently pump the soft-x-ray amplifier plasma
and allow generation at shorter wavelengths, we made use of a
tailored temporal pulse profile that consists of an 2-ns-long,
low-amplitude ramp that creates and ionizes the plasma and
a short-duration intense pulse that precedes the main peak of
the pulse as shown in Fig. 1(b). Hydrodynamic and atomic
physics plasma simulations show that the pump pulse profile,
consisting of a nanosecond ramp followed by two peaks
of picosecond duration, creates a plasma with an increased
density of Ni-like ions at the time of maximum temperature
that results in a larger gain coefficient over a temporally
and spatially enlarged region leading to a threefold increase
in the soft-x-ray laser output pulse energy. This increase in
pumping efficiency combined with the increased repetition rate
results in extremely high average power at these wavelengths
from a tabletop device. Using this approach, bright lasing
was also demonstrated at a number of wavelengths between
10.9 and 14.7 nm, including the high-repetition-rate, gain-
saturated operation of a λ = 11.9-nm laser from Ni-like Sn.
These results will enable technologic applications and basic
1050-2947/2014/89(5)/053820(7) 053820-1 ©2014 American Physical Society