Tuning the thermal conductivity of hydrogenated
porous magnesium hydride composites with the
aid of carbonaceous additives
L. Popilevsky
a,b
, V.M. Skripnyuk
a
, Y. Amouyal
a
, E. Rabkin
a,*
a
Department of Materials Science and Engineering, Technion-Israel Institute of Technology, Haifa 32000, Israel
b
Grand Technion Energy Program (GTEP), Technion-Israel Institute of Technology, Haifa 32000, Israel
article info
Article history:
Received 29 November 2016
Accepted 16 April 2017
Available online xxx
Keywords:
Hydrogen storage
Mg-based composites
MWCNTs
Microstructural characterization
Heat transfer
abstract
We synthesized solid porous pellets of the Mg-2 wt.% multiwall carbon nanotubes com-
posite and determined their thermal conductivity in partially hydrogenated state (80e90%
of their maximum hydrogen storage capacity). The thermal conductivities of the composite
pellets with carbon nanotubes were up to 20% higher than thermal conductivities of the
reference pellets of pure Mg prepared in a similar way. We demonstrated that the high
energy ball milling employed in the synthesis of the composites has destroyed the carbon
nanotubes and transformed them into chains of carbon nanoparticles of 20e30 nm in
diameter. The hydride phase grew preferentially along these chains, resulting in aniso-
tropic microstructure, with residual Mg phase forming an interpenetrating, percolating
network contributing to the long-range thermal transport. On the contrary, the residual Mg
formed isolated pockets in the reference pellets of pure Mg. Our work demonstrates that
anisotropic additives to the hydride forming metals can improve their thermal conduc-
tivity and hydrogen storage properties by changing the topology of the two-phase metal-
hydride microstructure.
© 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Introduction
Magnesium is considered as an attractive material for
renewable energy storage applications [1,2], thanks to its high
reversible hydrogen storage capacity (about 7.6 wt.% of H
2
)
and relatively low cost. However, its main drawbacks are slow
hydrogenation kinetics, low dissociation rate of hydrogen
molecules on the surface of Mg, high formation enthalpy of
MgH
2
(~75 kJ/mol H
2
at standard conditions), and high reac-
tivity toward oxygen.
Hydrogenation of metallic Mg begins from H
2
phys-
isorption on a surface followed by chemisorption during
which the H
2
molecule has to overcome an activation barrier
for its dissociation and formation of the hydrogen-metal bond
[3,4]. This is followed by atomic hydrogen penetration into the
metal and formation of the metal-hydrogen solid solution.
During the next step, nucleation of the magnesium hydride
phase (MgH
2
) starts as isolated sites on the surface of the
metal particle [5e7]. The shape of MgH
2
nuclei was reported to
be circular, suggesting isotropic growth [6,8]. These hydride
nuclei/colonies grow into the particle bulk until they impinge
on each other in such a way that the surface of the particles
becomes completely covered with hydride. It was shown that
MgH
2
nuclei impingement determines the final hydrogen
* Corresponding author. Fax: þ972 4 8295677.
E-mail address: erabkin@campus.technion.ac.il (E. Rabkin).
Available online at www.sciencedirect.com
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journal homepage: www.elsevier.com/locate/he
international journal of hydrogen energy xxx (2017) 1 e11
http://dx.doi.org/10.1016/j.ijhydene.2017.04.088
0360-3199/© 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Please cite this article in press as: Popilevsky L, et al., Tuning the thermal conductivity of hydrogenated porous magnesium hydride
composites with the aid of carbonaceous additives, International Journal of Hydrogen Energy (2017), http://dx.doi.org/10.1016/
j.ijhydene.2017.04.088