Research Article Adv. Mat. Lett. 2014, 5(7), 400-405 ADVANCED MATERIALS Letters
Adv. Mat. Lett. 2014, 5(7), 400-405 Copyright © 2014 VBRI press
www.amlett.com, www.vbripress.com/aml, DOI: 10.5185/amlett.2014.amwc.1038 Published online by the VBRI press in 2014
Development of nanocomposites based on
polypyrrole and carbon nanotubes for
supercapacitors
Ritu P. Mahore
1
, Devendra K. Burghate
1
, Subhash B. Kondawar
2*
1
Department of Physics, Shri Shivaji Science College, Nagpur 440015, India
2
Department of Physics, Polymer Nanotech Laboratory, RTM Nagpur University, Nagpur 440033, India
*
Corresponding author. Tel: (+91) 712-2042086; E-mail: sbkondawar@yahoo.co.in
Received: 08 October 2013, Revised: 30 November 2013 and Accepted: 22 December 2013
ABSTRACT
Supercapacitors are recognized as one of the most promising energy storage devices for a wide range of civilian and
military applications in electric vehicles, uninterruptible power supplies. Conducting polymer nanocomposites are new
functional materials suitable for supercapacitors due to synergistic effect of individual components. In present work,
polypyrrole/CNT nanocomposites have been prepared by an in-situ chemical polymerization method and studied for
supercapacitor. CNTs were well functionalized using 3:1 ratio of H
2
SO
4
and HNO
3
before polymerizing the pyrrole.
Analytical techniques such as SEM, UV-VIS and FTIR were used to characterize the synthesized materials. The SEM
images reveal that the materials have rough and granular morphology. The composites showed good interaction based on
the shift to longer wavelengths in the electronic transition, indicating the interaction between PPy and functionalized CNTs
as observed in their UV-VIS and FTIR spectra. The electrochemical performance was evaluated by using cyclic
voltammetry (CV) in 1M Na
2
SO
4
electrolyte and specific capacitance was obtained at 0.5 V/s for pure polypyrrole and
PPy/CNT nanocomposites. Nanocomposite showed the enhanced electrochemical performance as compared to that of pure
polypyrrole. The specific capacitance obtained at the scan rate 0.5V/s was found to be 0.825 F/cm
-2
for pure polypyrrole and
1.0619 F/cm
-2
for PPy/CNT nanocomposite material respectively, indicates that PPy/CNT nanocomposite is suitable
material as electrode for supercapacitor as compoared to pure polypyrrole. Copyright © 2014 VBRI press.
Keywords: Supercapacitor; polypyrrole; carbon nanotubes; cyclic voltammetry.
Ritu P. Mahore is working as Project
Fellow under Major Research Project funded
by UGC, New Delhi, in Department of
Physics, Shri Shivaji Science College,
Nagpur, India. She has obtained her master’s
degree in Physics from Rashtrasant Tukadoji
Maharaj Nagpur University, Nagpur, India.
She has registered for Ph.D. under the
supervision of Dr. D. K. Burghate and co-
supervision of Dr. S. B. Kondawar. Her
research interest includes the study of electrochemical performance of
ternary conducting polymer nanocomposites based on carbon nanotubes
for Supercapacitors.
Devendra K. Burghate is currently working
as Principal in Shri Shivaji Science College,
Nagpur, India. He did Ph.D. from
Department of Physics, Sant Gadge Baba
Amaravati University, Amaravati, India. His
main research activities include the study of
electrical properties of glasses. His current
research is focused on conducting polymer
nanocomposites for supercapacitors. He has published more than 30
research articles in journals of international repute. He has completed
two research projects funded by UGC, New Delhi (India).
Subhash B. Kondawar is currently working
as Professor in Department of Physics,
Rashtrasant Tukadoji Maharaj, Nagpur
University, Nagpur, India. He did Ph.D. from
Department of Physics, Institute of Science,
Nagpur, India. His main research activities
include the synthesis of advanced materials at
nanoscale and conducting polymer
nanocomposites. His current research is
focused on fabrication of electrospun
nanofibers of conducting polymers and nanocomposites for gas sensors,
biosensors and supercapacitors. He has published more than 35 research
articles in journals of international repute. He has completed three
major research projects funded by UGC, New Delhi (India).