Anal. Chem. Lett. 2022, 12, 266-282
DOI: 10.1080/22297928.2021.2021110
© 2022 Har Krishan Bhalla & Sons
Binding and Photocleavage Studies of Ru (II) Polypyridyl
Complexes with DNA: An In Silico and Antibacterial activity
Navaneetha Nambigari
1,2
*, Aruna Kodipaka
1
, Ravi Kumar Vuradi
2
,
Praveen Kumar Airva
3
and Satyanarayana Sirasani
2
*
1
Department of Chemistry, University College of Science, Osmania University,
Saifabad, Hyderabad-500004, Telangana, India
2
Department of Chemistry, University College of Science, Osmania University,
Tarnaka, Hyderabad-500007, Telangana, India
3
Department of Biotechnology, Sri Satya Sai University of Technology & Medical
Sciences, Opp. Oilfed Plant, Bhopal- Indore Road, Sehore-66001, Madhya
Pradesh, India
* Corresponding Authors: nitha379@gmail.com (Navaneetha Nambigari)
ssnsirasani@gmail.com (Satyanarayana Sirasani)
Supplementary Information
Experimental
All the Reagents and solvents of analytical
grade were used as received unless otherwise
stated. 1, 10-Phenanthroline monohydrate
(phen), 2,2’-bipyridine (bpy),4,4’-dimethyl-
2,2’-bipyridine (dmb), and 4,4’-dimethyl-1,10
orthophenonthroline (dmp) were procured
from Merck. Calf thymus DNA (CT-DNA) was
purchased from Aldrich, Super coiled pBR322
plasmid DNA (stored at 20ºC) from Fermentas
Life Sciences and was utilized as it is. Agarose
gel was bought from Genei. Ultrapure Milli-Q
water (18.2mX) was used in all experiments.
The binding afnity of metal complex for CT-
DNA was calculated in tris (hydroxymethyl)
amino methane, Tris–HCl bufer (5 m.mol Tris-
HCl, 50 mM NaCl, pH 7.2). The DNA, free of
protein was observed at an absorbance of 260 and
280 nm and a concentration of DNA per nucleotide
at a molar extinction Coefcient of 6600 M
-1
cm
-1
was determined spectrophotometrically
1,2
. Stock
solutions of DNA were kept at 40ºC and were put
to use in less than four days. The stock solutions
of concentrated metal complexes (calculated
amount) were made in DMSO, and were further
diluted to the requisite concentrations with
complimenting bufers for every experiment.
The UV-Vis spectra were recorded on
Shimadzu UV-2600 spectrophotometer. For
recording the luminescence spectral data for
determining the binding constants, Cary Eclipse
instrument serial number (MY12400004)
Spectrofuorometer was employed. IR spectra
were captured on a PerkinElmer 1605 Fourier
transform IR spectrometer using KBr disks.
1
H and
13
C NMR spectra were recorded by
using a Bruker 400-MHz spectrometer with
dimethyl-d6 sulfoxide (DMSO-d6) as the
solvent and tetramethylsilane as the internal
standard at room temperature. Elemental
microanalysis (C, H, and N) was performed
by using PerkinElmer 240 elemental analyzer.
Mass spectra were recorded with a Quattro LC
triple quadrupole mass spectrometer fortifed
with the Mass Lynx software program (Micro
mass, Manchester, UK)
3
.
i