Vol.:(0123456789)
Environmental Science and Pollution Research
https://doi.org/10.1007/s11356-024-33141-z
INTEGRATIVE APPROACH TO VARIOUS ENVIRONMENTAL TOXINS: EFFECTS
AND INTERACTIONS
Assessing metal(loid)s‑Induced long‑term spatiotemporal health risks
in Coastal Regions, Bay of Bengal: A chemometric study
Shammi Aktar
1
· Abu Reza Md. Towfiqul Islam
1,2
· Md Yousuf Mia
1
· Jannatun Nahar Jannat
1
· Md Saiful Islam
3
·
Md Abu Bakar Siddique
4
· Md Abdullah Al Masud
5
· Abubakr M. Idris
6,7
· Subodh Chandra Pal
8
·
Venkatramanan Senapathi
9
Received: 29 November 2023 / Accepted: 26 March 2024
© The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024
Abstract
Despite sporadic and irregular studies on heavy metal(loid)s health risks in water, fish, and soil in the coastal areas of the
Bay of Bengal, no chemometric approaches have been applied to assess the human health risks comprehensively. This
review aims to employ chemometric analysis to evaluate the long-term spatiotemporal health risks of metal(loid)s e.g.,
Fe, Mn, Zn, Cd, As, Cr, Pb, Cu, and Ni in coastal water, fish, and soils from 2003 to 2023. Across coastal parts, studies
on metal(loid)s were distributed with 40% in the southeast, 28% in the south-central, and 32% in the southwest regions.
The southeastern area exhibited the highest contamination levels, primarily due to elevated Zn content (156.8 to 147.2
mg/L for Mn in water, 15.3 to 13.2 mg/kg for Cu in fish, and 50.6 to 46.4 mg/kg for Ni in soil), except for a few sites in
the south-central region. Health risks associated with the ingestion of Fe, As, and Cd (water), Ni, Cr, and Pb (fish), and
Cd, Cr, and Pb (soil) were identified, with non-carcinogenic risks existing exclusively through this route. Moreover, As,
Cr, and Ni pose cancer risks for adults and children via ingestion in the southeastern region. Overall non-carcinogenic
risks emphasized a significantly higher risk for children compared to adults, with six, two-, and six-times higher health
risks through ingestion of water, fish, and soils along the southeastern coast. The study offers innovative sustainable
management strategies and remediation policies aimed at reducing metal(loid)s contamination in various environmental
media along coastal Bangladesh.
Keywords Chemometric technique · Heavy metal(loid)s · Human health risks · Data modelling · Coastal Bangladesh
Introduction
In recent decades, exponential population and wealth
growth has led to an increase in metal(loid)s contamination
in environmental compartments such as water, fish, soil,
and sediment (Ahmed et al. 2021a, b; Rakib et al. 2022a, b;
Hoque et al. 2022; Islam et al. 2020, 2023a; Ustaoglu and
Islam 2020). Therefore, rivers and oceans are particularly
vulnerable to aquatic systems due to urban, industrial,
and agricultural wastes. Metal(loid)s introduced to
aquatic environments generally accumulate in the bottom
sediments of rivers and oceans and play an important
role in the overall processes and biomagnification by
fish and other aquatic biota (Acharjee et al. 2022; Haq
et al. 2022). Like marine waters, terrestrial ecosystems
such as soil are also contaminated by hazardous metals,
a concern for scientists. Due to their ubiquity, trace
toxicity, bioaccumulation, and persistence, elevated
trace metals have been observed in soil–plant systems,
making soil contamination with metal (loids) a global
concern (Sarker et al. 2020a; Nguyen et al. 2020). Soil
is a biological buffer and geochemical sink for harmful
metals, transporting them to the atmosphere, hydrosphere,
and biota. Therefore, assessing the toxicity of metal(loid)
s in environmental compartments is very important to
reduce the toxic effects on the ecosystem.
Heavy metal(loid)s such as As, Ni, Cu, Zn, As, Cd, Pb,
and Cr are the most harmful toxins in the environment
worldwide and cause poisoning symptoms in all kinds of
living organisms, including humans (Hossain et al. 2020;
Responsible Editor: Luke Mosley
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