Sample Preparation Based on Dynamic
Ion-Exchange Solid-Phase Extraction for GC/MS
Analysis of Acidic Herbicides in Environmental
Waters
Nanqin Li and Hian Kee Lee*
Department of Chemistry, National University of Singapore, 3 Science Drive 3, Republic of Singapore 117543
The newly established enrichment technique, dynamic
ion-exchange solid-phase extraction (DIE-SPE), was stud-
ied for sample preparation for GC/MS analysis of 16
acidic herbicides in environmental waters. C
18
bonded
silica was the solid-phase material used. The optimal
sample pH was weakly acidic to neutral. However, for
common tap water and surface water, which run pH 6-9,
all the acidic herbicides except for Chloramben could be
effectively extracted from a sample of 1000-mL volume
without pH adjustment. The humic acid could be concur-
rently extracted from water, but most of it was separated
from the sample by using 3 mL of 10% methanol in
acetone as the eluent, which would completely elute the
analytes and leave a large part of the humic acid on the
cartridge. The selective elution reduced the interference
of humic acid and made the DIE-SPE an effective ap-
proach for the analysis of the acidic herbicides in surface
water. Comparing DIE-SPE with conventional reversed-
phase SPE (RP-SPE), the former gave higher recoveries
for the acidic herbicides and was less affected by sample
matrixes. A tandem-cartridge system combining RP- and
DIE-SPE in sequence was set up for the simultaneous
isolation of the acidic herbicides and removal of the
interfering substances. Despite some minimal retention
on the upper RP-SPE cartridge, most of the acidic
herbicides could be extracted on the lower DIE-SPE
cartridge with recovery over 80% except for Chloramben
(50%), fenoprop (73%), MCPB (67%), and 2,4-DB (70%)
when a 500-mL aqueous sample of pH 9.5 was percolated
through the tandem-cartridge system. The effectiveness
of the system in removing the long carbon chain fatty acids
as well as the basic and neutral organic interfering
substances from the sample was also demonstrated.
Acidic herbicides are mainly chlorophenoxy acids and related
compounds which are widely used in agriculture and forestry for
weed control. When released to the global environment, they may
generate certain toxicological effects on human beings and aquatic
life. EPA method 515.1 for acidic herbicides in drinking water
makes use of liquid-liquid extraction (LLE) followed by gas
chromatography-electron capture detector (GC-ECD).
1
Solid-phase
extraction (SPE) with adsorbent materials of ion exchangers,
2-6
reversed-phase bonded silica,
7-12
polymers,
13-16
and graphitized
carbon black (GCB),
17-20
has been widely investigated for sample
preparation of the acidic herbicides in water prior to chromato-
graphic determination.
Of the numerous organic pollutants, the acidic herbicides are
among those most compatible to SPE instead of conventional LLE
as the sample preparation technique for various environmental
waters. This is because, in common water matrixes, those acidic
herbicides are ionized and show a low tendency of adsorption on
the surface of glassware. Free filtration is possible before the
sample is applied to the SPE cartridge or disk and clogging of
the adsorbent bed can therefore be avoided, which is often the
problem with SPE methods for surface waters. For multiresidue
analysis of the acidic herbicides, there are two practical problems
for the existing SPE techniques. First, the hydrophilic acidic
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10.1021/ac991410c CCC: $19.00 © 2000 American Chemical Society Analytical Chemistry, Vol. 72, No. 14, July 15, 2000 3077
Published on Web 06/06/2000