Ganguly and Debnath, Med chem 2014, 4:8
DOI: 10.4172/2161-0444.1000194
Research Article Open Access
Med chem
ISSN: 2161-0444 Med chem, an open access journal
Volume 4(8): 558-568 (2014) - 558
Molecular Docking Studies and ADME Prediction of Novel Isatin Analogs
with Potent Anti-EGFR Activity
Swastika Ganguly* and Biplab Debnath
Department of Pharmaceutical Science and Technology, Birla Institute of Technology, Ranchi, India
*Corresponding author: Swastika Ganguly, Associate Professor, Department of
Pharmaceutical Sciences and Technology, Birla Institute of Technology, Ranchi,
India, Tel: 09431327042; E-mail: swastikaganguly@bitmesra.ac.in
Received May 24, 2014; Accepted July 25, 2014; Published July 28, 2014
Citation: Ganguly S, Debnath B (2014) Molecular Docking Studies and ADME
Prediction of Novel Isatin Analogs with Potent Anti-EGFR Activity. Med chem 4:
558-568. doi:10.4172/2161-0444.1000194
Copyright: © 2014 Ganguly S, et al. This is an open-access article distributed
under the terms of the Creative Commons Attribution License, which permits
unrestricted use, distribution, and reproduction in any medium, provided the
original author and source are credited.
Keywords: Cancer; Isatin; Epidermal growth factor receptor (EGFR);
Tyrosine kinase (TK); Docking; ADME
Introduction
Cancer is defined as a group of diseases characterized by
uncontrolled growth, and the spread of abnormal cells which if leſt
untreated may lead to death [1]. Cancer continues to be a major health
problem worldwide and more than ten million new cancer cases occur
annually, roughly half of which is prevalent in the developed countries,
and the disease causes over six million deaths a year [2].
Till date chemotherapy has been the mainstay of cancer therapy.
However the use of available chemotherapeutics is oſten limited mainly
due to undesirable side effects which include bone marrow depression,
alopecia, drug-induced cancer, hepatotoxicity, along with a limited
choice of available anti-cancer drugs [3].
Angiogenesis involves the proliferation of endothelial cells (ECs)
in response to specific growth stimuli such as vascular endothelial
growth factor (VEGF) of basic fibroblast growth factor (bFGF). Each
step of the process is controlled by these regulatory growth factors that
stimulate or inhibit angiogenesis. However, these control mechanisms
are oſten disordered in several pathologic diseases including cancer.
e growth and maintenance of solid tumors are highly dependent on
neovascularization and can be regulated by compounds that interfere
with either the stimulation or proliferation of ECs [4].
Angiogenesis has been intensely investigated as an attractive cancer
therapeutic target during the last decade as angiogenesis is the first
rate-limiting step for tumor cells to metastasize and is also essential for
cancer growth [1].
Some important receptors involved in angiogenesis have been
identified, including vascular endothelial growth factor receptor
(VEGFR), epidermal growth factor receptor (EGFR), and several
others. ese growth factor receptor kinases play important roles in
the development, progression, aggressiveness, and metastasis of many
solid tumors, such as non small cell lung cancer (NSCLC) , head and
neck cancers, and glioblastomas. Particularly, the involvement of the
EGFR family of tyrosine kinases in cancer proliferation suggests that
an inhibitor which blocks the tyrosine kinase activity of the entire
EGFR family could have significant therapeutic potential [5]. It is a
transmembrane receptor protein comprising of four homologs i. e.
EGFR/ErbB1/HER1, HER2/ Neu/ErbB2, HER3/ErbB3 and HER4/
ErbB4.
e isatin pharmacophore has attracted, and still attracts, much
attention from medicinal chemists because of its structural resemblance
to various moieties present in vitamins, proteins and nucleic acids.
Isatin moieties are of great importance in their biological as well as
synthetic approach of medicinal chemistry. From worldwide reported
literature, the various derivatives of isatin are known to possess a range
of biological properties including antibacterial and antifungal [6-10],
antiviral [11-13], anti-HIV [14,15], antiglycation [16], anticonvulsant
and sedative-hypnotic [17,18], anti-inflammatory [19] activities.
Various isatin derivatives have been reported to possess cytotoxic
activity [20-23]. us isatin is a biologically validated starting point for
the design and synthesis of chemical libraries directed at these targets
[24].
In recent years, rational drug design has become prevalent widely
in the pharmaceutical industry. is involves the use of computational
methods which are simple, non-expensive and speed up the process of
designing novel and potent molecules with desired biological activity.
Docking is a rational approach to drug design which seeks to predict
the structure and binding free energy of a ligand-receptor complex
given only the structures of the free ligand and receptor [25]. e setup
for a ligand docking approach requires the following components: A
target protein structure with or without a bound ligand, the molecules
of interest or a database containing existing or virtual compounds
for the docking process, and a computational framework that allows
the implementation of the desired docking and scoring procedures.
Docking accuracy reflects an algorithm’s ability to discover a
conformation (pose) (http://poseview. zbh. uni-hamburg. de) and
alignment of a ligand relative to a cognate protein that is close to that
experimentally observed and to recognize the pose as correct. Scoring
is the identification of the correct binding pose by its lowest energy
value, and the ranking of protein-ligand complexes according to their
binding affinities [26]. Molecular docking is oſten used in virtual
screening methods [27] whereby large virtual libraries of compounds
Abstract
Molecular docking studies were performed on 144 newly designed isatin analogs by using Glide v 5. 0 on the active
site of five crystal structures of EGFR enzymes (PDB ID 2J5F, 2ITW, 2ITY , 2ITX and1M17) to study the binding mode
of these analogs. Binding mode analysis of the compounds with the highest docking scores (-8. 31, -5. 90, -7. 16,
-6. 395 and -8. 14) was carried out and were compared with that of the co crystallized ligands DJK_3021_A, AFN
941
,
irressa, AMP-PNP and AQ4 in the active sites of 2J5F, 2ITW, 2ITY, 2ITX and 1M17 respectively. ADME properties of
all the newly designed isatin analogs 1-144 was calculated by Qik Prop v3. 0. All the designed compounds were found
to exhibit lead like properties from the calculated ADME properties.
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ISSN: 2161-0444
Medicinal chemistry