Chemistry
Volume 14 Issue 1 Version 1.0 Year 2014
Type : Double Blind Peer Reviewed International Research Journal
Publisher: Global Journals Inc. (USA)
Online ISSN: 2249-4626 & Print ISSN: 0975-5896
Analysis by GC-MS of an Aza-Michael Reaction Catalyzed by
CALB on an Orbital Shaker and under Microwave Irradiation
By Sandra S. Ribeiro, Marciana P. Uliana, Timothy J. Brocksom
& André L. M. Porto
Universidade De São Paulo, Brazil
Abstract- In this study, aza-Michael reactions between 1- phenylmethanamine and
α,β-unsaturated cyclohexenones were investigated, using lipase from Candida antarctica. The
reactions were performed in various organic solvents (CH
2
Cl
2
, hexane, MeOH, toluene, THF)
under mild conditions, with orbital shaking and microwave irradiation. The reactions showed
good results in the presence of CALB, yielding the Michael adducts and imines. The reaction
products were analyzed by GC-MS and in some cases it was found that the reverse aza-Michael
reaction had occurred.
GJSFR-B Classification :
AnalysisbyGC-MSofanAza-MichaelReactionCatalyzedbyCALBonanOrbitalhakerandunderMicrowaveIrradiation
Strictly as per the compliance and regulations of :
© 2014 Sandra S. Ribeiro, Marciana P. Uliana, Timothy J. Brocksom & André L. M. Porto. This is a research/review paper,
distributed under the terms of the Creative Commons Attribution-Noncommercial 3.0 Unported License http://creativecommons.
org/ licenses/by-nc/3.0/), permitting all non commercial use, distribution, and reproduction in any medium, provided the original
work is properly cited.
FOR Code: 100505, 250106
Global Journal of Science Frontier Research: B
Keywords: biocatalysis; amines; aza-Michael addition; enones; imines.