CHEMICAL ENGINEERING TRANSACTIONS
VOL. 56, 2017
A publication of
The Italian Association
of Chemical Engineering
Online at www.aidic.it/cet
Guest Editors: Jiří Jaromír Klemeš, Peng Yen Liew, Wai Shin Ho, Jeng Shiun Lim
Copyright © 2017, AIDIC Servizi S.r.l.,
ISBN 978-88-95608-47-1; ISSN 2283-9216
Flammability Assessments of Sonication Process in
Organic Mixture
Nur Amira Hasnul Hadi
a
, Arshad Ahmad*
,b
, Tuan Amran Tuan Abdullah
b
,
Adnan Ripin
b
a
Faculty of Chemical & Energy Engineering, Universiti Teknologi Malaysia, 81310 Johor Bahru, Malaysia
b
Centre of Hydrogen Energy, Institute of Future Energy, Universiti Teknologi Malaysia, 81310 Johor Bahru, Malaysia
arshad@cheme.utm.my
The prospect of sonication phenomenon in facilitating separation of azeotropic mixtures calls for more detailed
study towards developing an intensified distillation system. One important element that require in depth
consideration is safety since ultrasound is a potential ignition source with a low threshold value of 1 mW/mm
2
.
In this study, the aim is to investigate the potential of fire hazards that may be introduced by sonication when
used in the environment of flammable organic liquid. Simulation study in MATLAB programming environment
is carried out based on a mathematical model developed using first principle. Simulations of bubble conditions
covering its whole life cycle regimes are carried out and validated with experimental works. Evaluation is
made for an extreme condition where the ultrasonic waves are focused directed towards a stainless steel
target material immersed in ethanol-water mixture. As sonication occurs, bubbles form slowly by rectified
diffusion process with radius of 6 μm, and move toward the metal target. The experimental results revealed
that cavitation bubbles filled with explosive vapor are not ignited. This is consistent with the simulation study
where the maximum energy released during the bubble collapse is found to be small, which is 0.19267 pJ
compared to minimum ignition energy of the liquid at 0.23 mJ. This concludes that the focused ultrasound
wave in organic liquid does not trigger ignition, thus suggesting the ultrasonic distillation system is potentially.
1. Introduction
In recent years, separation of liquid mixtures has become one of the most important tasks in process industry.
From all separation technique available, distillation has been the most common method used. Because
distillation offers many processing advantages and mostly used, it still remain as the preferred process. For
mixtures that have azeotrope, separation process must have a specially chosen chemical to eliminate the
azeotropes points, namely entrainer (Ripin et al., 2009). Since azeotropic mixture could not be separated
using conventional distillation, it requires a new method for the separation.
Over the last few years, a large number of scientists has been working on chemical intensification process
and has developed an interest in ultrasonic distillation (Stankiewicz and Moulijin, 2002). The uniqueness of
ultrasound is that it is only operated in the presence of liquid to transmit its energy to enhance the physical
and chemical change of a liquid medium. Acoustic cavitation is the major phenomena that arise from the
propagation of ultrasonic waves in liquid (Ashokkumar, 2011). Power of ultrasound enhances the chemical
and mechanical effect by the generation and destruction of cavitation bubbles occur during the process
(Contamine et al., 1994).
Growth and collapse of bubble in sonication has yield the energy transfer from ultrasonic transducer to the
vapour inside the bubble (Gong and Hart, 1998). During this time, extremely high pressure in orders of
hundreds of atmosphere and high temperature up to 5,000 K are generated inside the bubble. Since
ultrasound are considered to be an ignition source by International Standard, this separation method has
reported no explosion neither fire accident in conjunction to ultrasound. However, incendivity of acoustic
cavitation on vapour liquid equilibrium in ultrasonic distillation is not yet to be to be study. This present work is
undertaken to determine whether will sonication during ultrasonic distillation triggered ignition.
DOI: 10.3303/CET1756233
Please cite this article as: Hadi N.A.H., Ahmad A., Abdullah T.A.T., Ripin A., 2017, Flammability assessments of sonication process in organic
mixture, Chemical Engineering Transactions, 56, 1393-1398 DOI:10.3303/CET1756233
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