ABSTRACT: Steryl ester content of refined and interesterified
corn, soybean, and rapeseed oils has been measured via clean-
up on a short silica gel column, followed by high performance
liquid chromatography with evaporative light-scattering mass
detector. Chemical interesterification, catalyzed by sodium
methoxide, led to random positional distribution of fatty acids
in triacylglycerols and some increase in the steryl ester content
of all three oils. Enzymatic interesterification, catalyzed by the
immobilized lipase from Rhizomucor miehei (Lipozyme), re-
sulted in a distinct reduction in steryl ester content, but essen-
tially no alteration in positional distribution of fatty acids in tri-
acylglycerols occurred. Formation of steryl esters during chemi-
cal and enzymatic interesterification was also examined by
radioactive tracer technique with [4–
14
C]β-sitosterol added as
marker to refined rapeseed oil and measurement of the radioac-
tive steryl esters formed. Chemical interesterification of rape-
seed oil resulted in moderate formation (10% of total radioac-
tivity) of radioactive β-sitosteryl esters. Enzymatic interesterifi-
cation of the oil, catalyzed by Lipozyme, led to little formation
of radioactive β-sitosteryl esters, whereas with the lipase from
Candida cylindracea high proportions (>90% of total radioac-
tivity) of
14
C-labeled β-sitosteryl esters were formed.
JAOCS 74, 93–96 (1997).
KEY WORDS: Candida cylindracea lipase, chemical inter-
esterification, enzymatic interesterification, positional distribu-
tion of fatty acids, radioactive tracer technique, Rhizomucor
miehei lipase, β-sitosterol, steryl esters.
Sterols occur in plant oils partly as unesterified sterols and
partly as steryl esters of fatty acids, in addition to steryl gly-
cosides and esterified steryl glycosides (1,2). We have re-
cently developed a method for quantitative determination of
steryl esters in oils by clean-up on a short silica gel column,
followed by high-performance liquid chromatography
(HPLC) with detection by means of an evaporative light-scat-
tering mass detector (Ferrari, R., E. Schulte, and K.D.
Mukherjee, manuscript in preparation). The above method
was used to monitor changes in steryl esters in plant oils at
different stages of industrial refining (Ferrari, R., E. Schulte,
and K.D. Mukherjee, manuscript in preparation). Here we re-
port the alterations in steryl ester content of plant oils by in-
teresterification, e.g., chemical interesterification (random-
ization) catalyzed by sodium methoxide, and enzymatic in-
teresterification catalyzed by lipase from Rhizomucor miehei
(Lipozyme). Moreover, we report the formation of steryl es-
ters during chemical interesterification and enzymatic inter-
esterification of rapeseed oil, catalyzed by Lipozyme and the
lipase from Candida cylindracea, as monitored by a radioac-
tive tracer technique. [4–
14
C]β-Sitosterol was added as
marker to the oil, and the formation of radioactive steryl es-
ters during interesterification was followed.
EXPERIMENTAL PROCEDURES
Materials. Refined corn oil was a product of Rafinacoes de
milho Brasil Ltda. (São Paulo, Brazil), and soybean and rape-
seed oils were provided by Cocamar Ltda. (Maringá, Brazil).
Immobilized lipase from R. miehei (Lipozyme IM20, 25 batch
interesterification units/g) was a generous gift of Novo Nordisk
(Bagsvaerd, Denmark). Powdered lipase preparation from C.
cylindracea (syn. C. rugosa) with an activity of 850 U/mg was
purchased from Sigma (Deisenhofen, Germany). β-Sitosterol
and [4–
14
C]β-sitosterol (56 mCi/mmol) were products of
Sigma and Amersham (Braunschweig, Germany), respectively.
β-Sitosteryl oleate was prepared according to Gupta et al. (3).
All reagents and adsorbents were of analytical grade and pur-
chased from E. Merck (Darmstadt, Germany).
Chemical interesterification. Refined oil (10 g) and 15 mg
sodium methoxide were placed in a round-bottom flask, and
the mixture was stirred magnetically at 110˚C for 30 min
under vacuum generated by a water jet aspirator. The reaction
products were cooled to room temperature, dissolved in
hexane, and washed repeatedly with an aqueous 1% (wt/vol)
sodium chloride solution to remove the soaps completely. The
hexane solution of the interesterified product was dried over
sodium sulfate and stored refrigerated under nitrogen.
Copyright © 1997 by AOCS Press 93 JAOCS, Vol. 74, no. 2 (1997)
1
Part of doctoral thesis of Roseli Ap. Ferrari to be submitted to Faculdade de
Engenharia de Alimentos, Universidade de Campinas, Campinas, Brazil.
*To whom correspondence should be addressed at Institute for Biochemistry
and Technology of Lipids, H.P. Kaufmann-Institute, BAGKF, Piusallee 68,
D-48147 Münster, Germany.
Alteration of Steryl Ester Content and Positional Distribution
of Fatty Acids in Triacylglycerols by Chemical
and Enzymatic Interesterification of Plant Oils
1
R.Ap. Ferrari
a
, W. Esteves
b
, and K.D. Mukherjee
a,
*
a
Institute for Biochemistry and Technology of Lipids, H. P. Kaufmann-Institute, Münster, Germany,
and
b
Laboratory of Oils and Fats, University of Campinas, Campinas, Brazil