Vol.:(0123456789)
Polymer Bulletin
https://doi.org/10.1007/s00289-019-02947-0
1 3
ORIGINAL PAPER
Performance tendency and morphological investigations
of lignocellulosic tea/polyurethane bio‑composite
materials
Y. A. El‑Shekeil
1
· F. M. AL‑Oqla
2
· S. M. Sapuan
3,4
Received: 10 April 2019 / Revised: 14 June 2019 / Accepted: 7 September 2019
© Springer-Verlag GmbH Germany, part of Springer Nature 2019
Abstract
This work investigates the effect of reinforcing conditions at optimal processing
parameters on the morphological properties as well as the mechanical performance
of tea/polyurethane bio-composites. Various reinforcing conditions were designed
and prepared to reveal the performance tendency and effects of the reinforcing con-
ditions on several composites properties including tensile strength, tensile modulus,
elongation to break, in addition to the morphological characteristics of the bio-com-
posites. ASTM standards were considered in performing the performance testing of
the composites. Results have demonstrated that only tensile moduli were enhanced
with fiber loading, but tensile strength deteriorations occurred. Moreover, this work
investigates the similarity in trends for some mechanical behaviors of the compos-
ites. Similar trends in reducing the composites strengths as well as the composites
strains with increasing fiber loading were detected. This was an evidence of the
strong adhesion between the fiber and the polymer in the TWF/TPU composites,
which is not necessarily enhancing the composite strength. Such strong adhesion
was proved here not necessary to enhance the composite strength. However, the poor
filler dispersion due to excessive fiber loading leads to some agglomeration of the
fillers as observed by the scanning electron microscopy, which makes it suitable for
various industrial applications.
Keywords Bio-composites · Performance trends · Fracture · Thermoplastic
polyurethane · Mechanical properties · Lignocellulosic fibers
* F. M. AL-Oqla
fmaloqla@hu.edu.jo
Extended author information available on the last page of the article