THE ELECTRODEPOSITION OF Al-Cu ALLOYS FROM
ROOM-TEMPERATURE CHLOROALUMINATE ELECTROLYTES
G.R. Stafford, V.D. Jovic and T.P Moffat
Materials Science and Engineering Laboratory
National Institute of Standards and Technology
Gaithersburg, Maryland 20899, USA
Q. Zhu, S. Jones and C.L. Hussey
Department of Chemistry
University of Mississippi
University, Mississippi 38677, USA
ABSTRACT
The electrodeposition of Cu-Al alloys, as well as the underpotential
deposition (UPD) of A1 onto Cu(l 11), were investigated in acidic aluminum
chloride/1-methy 1-3-ethylimidazolium chloride ambient temperature molten
salt. It was shown that it is possible to produce Cu-Al alloy deposits at
potentials positive of that corresponding to the electrodeposition of bulk Al.
The onset of Al codeposition was found to occur at approximately 0.30 V
versus the A1(III)/A1 couple, and the Cu-Al alloy composition was found to
be independent of the Cu(I) concentration, reaching a maximum value of 43
% atomic fraction Al at 0 V. Alloy deposition potentials based on free
energy calculations are in good agreement with those observed
experimentally for Zn-Al, Cu-Al, Co-Al, and Fe-Al deposited at room
temperature and Ni-Al deposited at 150 °C from an aluminum
chloride/sodium chloride melt. Cyclic voltammograms recorded on Cu(l 11)
clearly indicate that UPD of Al commences at about 0.30 V vs. Al and is
characterized by two distinct surface processes. In-situ scanning tunneling
microscopy (STM) examination indicates that an ordered ad-layer appears
on the C u (lll) surface at potentials positive of the first UPD wave. A
possible model representing this structure corresponds to a layer of
tetrachloroaluminate ions, oxidatively adsorbed on the C u (lll) surface,
with the face of the tetrahedra adjacent to the copper surface.
INTRODUCTION
Aluminum alloys can be electrodeposited from chloroaluminate molten salts with the
addition of the solute metal ions to the electrolyte. This can be accomplished by either
anodic dissolution of the solute metal directly into the melt or by the addition of the
appropriate chloride salt. The formation of Al-transition metal alloys is also possible even
though the deposition potential of the transition metal may be several hundred millivolts
more positive than that of Al. The mechanism leading to the formation of these alloys is a
variant of underpotential deposition (UPD) phenomena whereby alloy formation proceeds
by co-deposition of Al during the mass-transport-limited electrodeposition of the
transition metal. Such interesting alloy formation has been demonstrated for Al-Ni (1)
from AlCl3:NaCl electrolyte as well as Al-Ni (2-4), Al-Co (5,6) and Al-Cu (7,8) from the
room-temperature chloroaluminates. In this article, we describe the electrodeposition of
Cu and the underpotential co-deposition of Al with Cu to form Cu-Al alloys from
solutions of Cu(I) in the Lewis acidic AlCl3-MeEtimCl melt. Alloy deposition potentials
independently derived from the free energy of alloy formation are compared to those
observed experimentally for several aluminum alloy systems. In addition we examine the
Proceedings of The Electrochemical Society, PV 1999-41, 535-548 (1999)
DOI: 10.1149/199941.0535PV © The Electrochemical Society
) unless CC License in place (see abstract). ecsdl.org/site/terms_use
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