Vol.:(0123456789) 1 3
Chemical Papers
https://doi.org/10.1007/s11696-018-0487-6
ORIGINAL PAPER
Study of the binding sites in the biomass of Aspergillus niger wild‑type
strains by FTIR spectroscopy
Katarína Gáplovská
1
· Alexandra Šimonovičová
2
· Radoslav Halko
3
· Lenka Okenicová
3
· Mária Žemberyová
3
·
Slavomír Čerňanský
4
· Paula Brandeburová
5
· Tomáš Mackuľak
5
Received: 19 December 2017 / Accepted: 25 April 2018
© Institute of Chemistry, Slovak Academy of Sciences 2018
Abstract
Fourier transform infrared (FTIR) spectroscopy studies were performed to confirm and to provide information on the identity
and binding characteristics of the chemical groups responsible for the binding of elements using Aspergillus niger (A. niger)
wild-type strains. Two absorption bands in the 3690–3615 and 2970–2895 cm
−1
regions can characterize stretching vibrations
OH and CH groups in fatty acids, respectively, and intensive bands around of 1600 cm
−1
and by 1048 cm
−1
correspond to
stretching vibrations of C=O groups of amides (amide I) or stretching vibrations ν(C–N). The FTIR results confirmed that
no extra differences between IR spectra of A. niger in raw biomass and in solid rest after extraction with chloroform were
observed. The small differences were observed in IR spectra of A. niger in chloroform after extraction.
Keywords Aspergillus niger · Bioaccumulation · Binding sites · FTIR spectroscopy · UV spectroscopy · Elemental analysis
Introduction
Microscopic filamentous fungi are ubiquitous and wide-
spread microorganisms that play an important role in bio-
degradation of organic material in the environment. How-
ever, living as well as non-living fungal biomass can be used
in sorption processes mainly due to unique composition of
its cell walls (Gow et al. 2017; Dhankhar and Hooda 2011;
Volesky 2003). This structural uniqueness of fungal cell
walls differs significantly among various fungal species as
well as fungal strains of the same species (Bowman and Free
2006). Thus, fungal metabolism and chemical composition
of fungal cells are strongly dependent on the studied fun-
gal strain and its original habitat affected by various envi-
ronmental factors (Zemberyova et al. 2014; Šimonovičová
et al. 2013). Fungal cell walls contain numerous quantities
of glycoproteins and polysaccharides, mainly glucan and
chitin, which can provide abundant functional groups (e.g.,
carboxyl, hydroxyl, sulphonate, phosphoryl, amido, amino,
and imidazole groups) for metal(loid) binding (Vendruscolo
et al. 2017; Horník et al. 2013; Chojnacka 2010). The strong
species and strain diversity and differences in chemical com-
position of fungal cell walls allow applying fungi in biosorp-
tion processes of both cationic and anionic contaminants
(Dadval and Mishra 2017; Gola et al. 2017; Rodríguez et al.
2013).
Bioprospecting and further application of such different
strains of the same species can be very beneficial for their
variable uses such as removal of potentially toxic metal(loid)
s from wastewaters. Moreover, filamentous fungi are applied
in a variety of industrial fermentation processes which can
serve as a rich source of biomass for metal(loid) removal.
Therefore, fungi can be considered as low-price biosorbent
with a high metal(loid)-binding capacity and selectivity for
metal(loid)s (Yang et al. 2017; Wang and Chen 2006).
* Paula Brandeburová
brandeburova.paula@gmail.com
1
Faculty of Natural Sciences, Institute of Chemistry,
Comenius University, Mlynská dolina CH-2, Ilkovičova 6,
842 15 Bratislava, Slovakia
2
Department of Soil Science, Faculty of Natural Sciences,
Comenius University, Mlynská dolina B-2, Ilkovičova 6,
842 15 Bratislava, Slovakia
3
Department of Analytical Chemistry, Faculty of Natural
Sciences, Comenius University, Mlynská dolina CH-2,
Ilkovičova 6, 842 15 Bratislava, Slovakia
4
Department of Environmental Ecology, Faculty of Natural
Sciences, Comenius University, Mlynská dolina B-2,
Ilkovičova 6, 842 15 Bratislava, Slovakia
5
Department of Environmental Engineering, Faculty
of Chemical and Food Technology, Slovak University
of Technology, Bratislava, Slovakia