ORIGINAL PAPER
Selection of thermotolerant Saccharomyces cerevisiae
for high temperature ethanol production from molasses
and increasing ethanol production by strain improvement
Sornsiri Pattanakittivorakul
.
Noppon Lertwattanasakul
.
Mamoru Yamada
.
Savitree Limtong
Received: 11 October 2018 / Accepted: 12 January 2019
© Springer Nature Switzerland AG 2019
Abstract A thermotolerant ethanol fermenting
yeast strain is a key requirement for effective ethanol
production at high temperature. This work aimed to
select a thermotolerant yeast producing a high
ethanol concentration from molasses and increasing
its ethanol production by mutagenesis. Saccha-
romyces cerevisiae DMKU 3-S087 was selected
from 168 ethanol producing strains because it
produced the highest ethanol concentration from
molasses at 40 °C. Optimization of molasses broth
composition was performed by the response surface
method using Box–Behnken design. In molasses
broth containing optimal total fermentable sugars
(TFS) of 200 g/L and optimal (NH
4
)
2
SO
4
of 1 g/L,
with an initial pH of 5.5 by shaking flask cultivation
at 40 °C ethanol, productivity and yield were 58.4 ±
0.24 g/L, 1.39 g/L/h and 0.29 g/g, respectively. Batch
fermentation in a 5 L stirred-tank fermenter with 3 L
optimized molasses broth adjusted to an initial pH of
5.5 and fermentation controlled at 40 °C and 300 rpm
agitation resulted in 72.4 g/L ethanol, 1.21 g/L/h
productivity and 0.36 g/g yield at 60 h. Strain DMKU
3-S087 improvement was performed by mutagenesis
using ultraviolet radiation and ethyl methane sul-
fonate (EMS). Six EMS mutants produced higher
ethanol (65.2 ± 0.48–73.0 ± 0.54 g/L) in molasses
broth containing 200 g/L TFS and 1 g/L (NH
4
)
2
SO
4
by shake flask fermentation at 37 °C than the wild
type (59.8 ± 0.25 g/L). Among these mutants, only
mutant S087E100-265 produced higher ethanol (62.5
± 0.26 g/L) than the wild type (59.5 ± 0.02 g/L) at
40 °C. In addition, mutant S087E100-265 showed
better tolerance to high sugar concentration, furfural,
hydroxymethylfurfural and acetic acid than the wild
type.
Keywords Ethanol fermentation ·
Thermotolerant yeast · Molasses · Mutagenesis ·
Ethyl methane sulfonate
Introduction
High temperature ethanol fermentation is required for
effective ethanol production in tropical countries that
have elevated temperatures throughout the year.
Fermentation at high temperature has several advan-
tages including rapid fermentation rate, reduction of
S. Pattanakittivorakul · N. Lertwattanasakul ·
S. Limtong (&)
Department of Microbiology, Faculty of Science,
Kasetsart University, Chatuchak, Bangkok 10900,
Thailand
e-mail: fscistl@ku.ac.th
M. Yamada
Applied Molecular Bioscience, Graduate School of
Medicine, Yamaguchi University, Ube,
Yamaguchi 755-8505, Japan
S. Limtong
Academy of Science, The Royal Society of Thailand,
Bangkok 10300, Thailand
123
Antonie van Leeuwenhoek
https://doi.org/10.1007/s10482-019-01230-6