CHEMICAL ENGINEERING TRANSACTIONS
VOL. 43, 2015
A publication of
The Italian Association
of Chemical Engineering
Online at www.aidic.it/cet
Chief Editors: Sauro Pierucci, Jiří J. Klemeš
Copyright © 2015, AIDIC Servizi S.r.l.,
ISBN 978-88-95608-34-1; ISSN 2283-9216
Modeling of Phase and Chemical Equilibria for Systems
Involved in Biodiesel Production
Larissa P. Cunico, Reginaldo Guirardello*
School of Chemical Engineering, State University of Campinas (UNICAMP), Av. Albert Einstein 500, 13083-852. Campinas-
SP. Brazil
guira@feq.unicamp.br
In recent years, the interest in the use of renewable energy has encouraged the growth of studies into
renewable sources, such as the production of biofuels. This work investigates the vapor-liquid equilibrium
(VLE), vapor-liquid-liquid equilibrium (VLLE) and liquid-liquid equilibrium (LLE) of binary, ternary, quaternary
and pseudo-quaternary systems using an optimization approach for components found in biodiesel
production, which consists in vegetable oils, fatty acids, esters and alcohols. A methodology has been
developed based on the Gibbs energy minimization and the discretization of the molar fraction domain, which
incorporates a thermodynamic model to describe the phase equilibria. This work used the Soave-Redlich-
Kwong equation of state (SRK-EOS) for phase equilibria calculation, where the compressibility factor was
used to determine the phase present in the system (liquid, vapor or supercritical fluid). The chemical and
phase equilibrium problem is solved using linear programming and satisfies the mass balance constraints. It
was found that the proposed methodology adequately represents the selected experimental data, with an
average absolute deviation of 1.31 % obtained.
1. Introduction
The most used energy sources worldwide are still non-renewable, such as oil, coal and natural gas. Factors
such as environmental problems encourage the growth of studies in renewable sources such as biofuels. In
large development, biodiesel has the main advantages: 1) It is biodegradable and non-toxic; 2) It contributes
to the reduction of greenhouse gases, emissions of particulate matter and acid rain. The biodiesel production
involves a number of processing steps that require knowledge of chemical or phase equilibrium.
When a system is in equilibrium, the Gibbs energy has a minimum value for a given pressure and
temperature. The calculation of the correct number of phases in equilibrium and its composition can be divided
in two mainly categories: through the equation-solving approach for searching same fugacity or chemical
potential in all the present phases in equilibrium, or through the direct minimization of the Gibbs energy (Teh
and Rangaiah, 2002). The first approach solves the necessary conditions to guarantee chemical equilibrium,
but only one solution minimizes the Gibbs energy and satisfies the second law of thermodynamics.
Considering the minimization of Gibbs energy, a common problem observed is the convergence in a global
solution and a good estimate of the composition as a starting point is required.
This work presents a linear program model formulation for phase and chemical equilibria calculation in
quaternary and pseudo-quaternary systems, based on a discretization of the molar fraction domain. The
proposed approach can be applied to any thermodynamic model such as equations of state or excess Gibbs
energy models. However, in this work, the equation of state of Soave-Redlich-Kwong (SRK-EOS) with the
mixing rule of van der Waals two adjustable parameters (VDW-2) was employed. The use of this equation of
state allows the calculation of both vapor-liquid equilibrium in elevated conditions of pressure and
temperature, vapor-liquid in lower conditions of pressure and temperature, and liquid-liquid equilibrium. In the
second part of this work, the performance of the proposed method in predicting phase and chemical
DOI: 10.3303/CET1543310
Please cite this article as: Cunico L., Guirardello R., 2015, Modeling of phase and chemical equilibria for systems involved in biodiesel
production, Chemical Engineering Transactions, 43, 1855-1860 DOI: 10.3303/CET1543310
1855