Cobalt Nanostructured Coatings for Methanol
Anodic Oxidizing
Maryna Ved*, Nikolay Sakhnenko and Tatiana Nenastina
National Technical University, Ukraine
Introduction
Eco-friendly Fuel Cells (FC), Solar Cells (SC) are among the promising renewable energy
sources, however, the high cost of the noble metal electrodes prevents their dissemination
and widespread use. Development of FC, SC and various Red-ox Flow Batteries (RFB) needs
to create effective catalytic electrodes based on the transition metals. Among the most
important requirements to electrode materials are chemical stability of the surface and
inactivity to technological environment components; wide window of polarization potentials,
in which electrode stays inactive; high selectivity and catalytic activity toward main electrode
reactions; significant specific surface area. Even brief review gives an impression that in
scientific literature for the last years there are too few publications on electrode materials
on the basis of hi-tech materials, such as nanostructured and nanocrystalline materials based
on the corrosion resistant amorphous metal alloys (metal glass), or nanostructured deposits
by synergistic alloys [1-3]. The most efficient directions of catalytic materials synthesis are
electrochemical technologies that provide flexibly control the composition, the deposition
rate, the state of the surface, by varying the electrolyte nature and polarization mode [4-6].
Because of this it is possible to fabricate the deposits with desirable functional properties
(synergistic or additive) [7-10].
Methods
Alloys Co-Mo-W(Zr) were deposited onto the steel substrate from a citrate-diphosphate
bath in pulse mode [7,9]. The chemical composition of the coatings was determined by
energy dispersive X-ray spectroscopy (EDS) on an Oxford INCA Energy 350 electron probe
microanalysis integrated into the system of the SEM. The surface morphology of the deposits
was studied with a Zeiss EVO 40XVP scanning electron microscope (SEM). The surface
roughness was evaluated by the contact method on 10×10×2mm samples with an NT-206
scanning probe AFM microscope (CSC cantilever B as probe, probe tip radius 10nm). The
AFM results are reflected at the Figure 1. The structure of the deposits was examined by X-ray
diffraction analysis using a diffractometer (DRON-2.0) in the emission of iron anode and CuKα
radiation. Electro catalytic properties of coatings were studied in model reaction of methanol
electrooxidizing in alkali medium using Cyclic Voltammetry (CVA) technique [1].
Result and Discussion
Structure of the ternary alloys was found to be amorphous-crystalline (Figure 1), and
coherent-scattering region size was of 2-8nm. Co-Mo-W coatings contain intermetallic phases
Co
7
W
6
, and Co
7
Mo
3
(Figure 2a), and Co
3
Mo and Co
7
Mo
6
ones are found in the structure of Co-Mo-
Zr deposits (Figure 2b). Analysis CVA obtained at the Co-Mo-Zr coated electrode polarization
in methanol containing alkaline solution shows the ratio of reverse and direct current to be
Crimson Publishers
Wings to the Research
Mini Review
*Corresponding author: Maryna Ved,
National Technical University, Ukraine
Submission: September 13, 2019
Published: November 21, 2019
Volume 1 - Issue 3
How to cite this article: Maryna Ved*, Ni-
kolay Sakhnenko and Tatiana Nenastina .
Cobalt Nanostructured Coatings for Meth-
anol Anodic Oxidizing. Determinations
anomed Nanotechnol.
1(3). DNN.000514.2019.
DOI: 10.31031/DNN.2019.01.000514
Copyright© Maryna Ved, Kanwal Iqbal,
This article is distributed under the terms
of the Creative Commons Attribution 4.0
International License, which permits
unrestricted use and redistribution
provided that the original author and
source are credited.
1 Determinations in Nanomedicine & Nanotechnology
Abstract
A. Co-Mo-W(Zr) electrolytic alloys of both amorphous & crystalline structure were deposited in pulse
mode.
B. Above alloys exhibit catalytic activity in methanol electrooxidizing in alkali media.
C. Ternary coatings were shown to be may be cycled and thus utilized as electrode materials for fuel cells.
ISSN : 2832-4439