16
P.P. Lizymol / Trends Biomater. Artif. Organs, 36(1), 16-20 (2022)
*Coresponding author
E-mail address: lizymol@sctimst.ac.in (Dr. P.P. Lizymol)
X-ray Microcomputed Tomography (μCT) Studies of a New Low
Shrinkage Visible Light Cure Dental Composite (Ormo48): Effects
of Thermal Cycling on Physical Properties
P.P. Lizymol
Division of Dental Products, Biomedical Technology Wing, Sree Chitra Tirunal Institute for Medical Sciences and Technology, Poojappura, Thiruvananthapuram 695012, India
Received: 9 December 2021
Accepted: 25 December 2021
Published online: 22 January 2022
Keywords: dental composite, thermal
cycling, microhardness, microcomputed
tomography, diametral tensile strength,
Ormo48
This study investigated the effects of cyclic temperature changes on internal porosity generation, diametral tensile
strength (DTS) and surface hardness of an experimental organically modified ceramic composite (Ormo48) dental
restorative material with superior shrinkage characteristics. In this study, a novel organically modified ceramic resin
has been synthesized and used as the binding resin along with quartz filler for composite preparation. The
photocured composite samples were subjected to thermal cycling up to 2000 cycles from 5
o
C to 55
o
C in a dental
thermal cycler and the properties were evaluated as per ISO and ADA standards. MicroCT analysis was carried out
to find the effect of cyclic temperature changes on the porosity and internal structure of the cured restorative.
Statistical evaluation using analysis of variance (ANOVA single factor) showed that thermal cycling up to 500 cycles
resulted in significant decrease in DTS whereas no significant change in surface hardness was noticed. With thermal
cycling both pore size and pore volume of cured Ormo48 increased as evidenced by microCT results.
© (2022) Society for Biomaterials & Artificial Organs #20056222
Original Article
Introduction
Polymer based composite materials used in dentistry for direct
restorative purpose are mostly in situ polymerizable methacrylate
based thermoset materials, which have been widely acceptable due
to their better aesthetic, and concerns about dental amalgam
fillings [1] and became the good choice of dentists to satisfy the
demands of patient’s aesthetics. Like any other composite system,
a dental composite is a material system composed of two or more
constituents mainly an organic resin and inorganic filler, which are
essentially insoluble in each other. The major components of
restorative materials are the inorganic filler or combination of
different fillers forming hybrid system. The filler particles used for
the dental composite preparation were commonly quartz, nano
silica or radiopaque glass alone or in combination.
The binding resin generally comprised of high molecular weight
dimethacrylates monomers including (bisphenol-A glycidyl
methacrylate) or urethane di/tetra methacrylates. Most current
research efforts are directed towards reducing polymerisation
shrinkage of the existing resin system by incorporating different
monomers as well as developing entirely new monomers include
ring-opening polymerisation, prepare analogues of BisGMA, use
of liquid crystalline monomers, thiol-ene reaction, bicycloacrylates,
siloranes, spiro orthocarbonates and organically modified ceramics
for dental composites [2-6].
The use of ring-opening polymerisation (ROP) could help
circumvent polymerisation shrinkage, since the polymerisation
reaction involves the breaking of a bond for every new bond
formed [1]. Radical ring-opening polymerisation, of
bicycloacrylates, is an example of monomer with low
polymerization shrinkage However, the polymers displayed a
greater water uptake, which limits its long-term strength [2-3].
Spiro orthocarbonates have shown reduced shrinkage because of
the double ring-opening polymerisation, with two bonds broken
for every new bond created, leading to volume expansion upon
polymerisation [4]. However, due to their poor curing
characteristics they have insufficient mechanical strength. A new
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