Trehalose (αDglucopyranosylαDglucopyra
noside), a nonreducing disaccharide, is present in var
ious organisms including bacteria, fungi, plants, and
mammals [1]. Trehalose is found in spores, in resting
cells, and in cells subjected to different forms of stress.
This universality is related to the unique ability of this
sugar to maintain the native state of membranes in con
ditions of high ionic strength, dehydration, elevated
temperature [15]. Many organisms can also use tre
halose as an exogenous source of carbon.
Certain grampositive and gramnegative bacteria
including Escherichia coli can grow using trehalose as the
only source of carbon at both low and high osmolarity,
when the sugar is synthesized and accumulated inside a
cell. It seems to be paradoxical: trehalose is cleaved as a
source of carbon and simultaneously it is synthesized as
an osmoprotector. For realization of these two pathways
bacteria have developed two different systems of trehalose
metabolism, one for high and the other one for low osmo
larity. The scheme of trehalose metabolism has been stud
ied in detail for E. coli [6]. Trehalose diffuses to the
periplasm through LamB pores. Under conditions of low
osmolarity, trehalose is transported through periplasm
membrane and simultaneously phosphorylated by
EIICB
Tre
(TreB) enzyme of the phosphotransferase sys
tem (PTS) using EIIA of glucose PTS (EIIA
Glc
) as phos
phoryl donor. In cytoplasm, trehalose6phosphate is
hydrolyzed to glucose and glucose6phosphate by the
enzyme trehalose6phosphate hydrolase (TreC). Free
glucose is phosphorylated by glucokinase, and glucose6
phosphate is subjected to glycolysis. At high osmolarity
both TreB and TreC are repressed. Trehalose is
hydrolyzed in periplasm to two glucose molecules by
periplasmic trehalase (TreA). The latter is activated in
turn at high osmolarity. Glucose is transported to the
cytoplasm through the phosphotransferase system of glu
cose. On the other hand, trehalose is synthesized at high
osmolarity by the enzymes trehalose6phosphate syn
thase (OtsA) and trehalose6phosphate phosphatase
(OtsB) using glucose6phosphate and UDPglucose as
the substrates.
The objective of this study was cloning of the gene
encoding the enzyme trehalose6phosphate hydrolase
from the thermophilic bacterium Bacillus sp. GP16, and
study of the principal enzymatic properties of this pro
tein. Here we determined the Michaelis–Menten con
stant as functions of pH, temperature, and ionic strength.
It should be noted that this enzyme is poorly studied bio
chemically, and the kinetic data in the literature are con
troversial. The expression and purification of the enzyme
from a thermophilic source was carried out for the first
time in this work.
Biochemistry (Moscow), Vol. 68, No. 9, 2003, pp. 10121019. Translated from Biokhimiya, Vol. 68, No. 9, 2003, pp. 12381246.
Original Russian Text Copyright © 2003 by Karelov, Krasikov, Surjik, Firsov.
00062979/03/68091012$25.00 ©2003 MAIK “Nauka / Interperiodica”
* To whom correspondence should be addressed.
Expression, Isolation, Purification, and Biochemical Properties
of Trehalose6phosphate Hydrolase from Thermoresistant Strain
Bacillus sp. GP16
D. V. Karelov, V. V. Krasikov, M. A. Surjik, and L. M. Firsov*
Konstantinov St. Petersburg Institute of Nuclear Physics, Russian Academy of Sciences, Gatchina 188350,
Leningrad Region, Russia; Email: lfirsov@mail.wplus.net
Received July 24, 2002
Revision received October 29, 2002
Abstract—Here we describe cloning, expression, and purification of the enzyme trehalose6phosphate hydrolase from ther
moresistant strain Bacillus sp. GP16. Principal biochemical properties of the enzyme at different pH and temperature values
were determined. Entropy and enthalpy of activation of the enzyme for substrates trehalose6phosphate and pnitrophenyl
glucoside were calculated, and the dependence of the kinetic parameters from ionic strength was established.
Key words: trehalose6phosphate hydrolase, cloning of a gene, gene expression, catalysis, temperature dependence, deter
mination of Michaelis constants