Original Article
CHIRAL SWITCHING CONTROL OF PHARMACEUTICAL SUBSTANCES
OLGA V. LEVITSKAYA , TATIANA V. PLETENEVA
*
, DARIA A. GALKINA , NADEZDA A. KHODOROVICH ,
ELENA V. USPENSKAYA , ANTON V. SYROESHKIN
Pharmaceutical and Toxicological Chemistry Department, RUDN University, 6 Miklukho-Maklaya St, Moscow-117198, Russian Federation
*Corresponding author: Tatiana V. Pleteneva;
*
Email: tvplet@mail.ru
Received: 29 Jan 2024, Revised and Accepted: 16 Mar 2024
ABSTRACT
Objective: The aim of this study was to demonstrate that chiral switching should be recognized as a widespread phenomenon that extends beyond
the production of pure enantiomeric drugs.
Methods: To investigate the optical activity of substances from various chemical classes, enantiomers of chiral compounds (Sigma-Aldrich, USA)
were chosen: valine and its racemic form (D-valine, L-valine, and racemic valine with optical purity ≥ 99%), L-ascorbic acid (content ≥ 99%),
carbohydrates (D-glucose, D-galactose, L-galactose, contents ≥ 99.5%). Solutions were prepared using deuterium-depleted water (DDW–"light"
water, D/H=4 ppm), natural deionized high-ohmic water (BD, D/H=140 ppm), and heavy water (99.9% D2O; Sigma-Aldrich). Optical activity was
measured using the Atago POL-1/2 polarimeter.
Results: One of the components in the racemic medication mixture can act as an inert agent, exhibit toxicity, or undergo undesirable
biotransformation mechanisms, resulting in the formation of products with unknown properties. It has been established that a change in the
deuterium/protium (D/H) ratio in water leads to a change in the equilibrium and kinetic characteristics of optically active compounds across
various chemical classes, such as amino acids, carboxylic acids, and carbohydrates. An inequality was observed in the absolute values of the optical
rotation of the L-and D-isomers of valine and galactose, depending on the D/H isotope ratio. The impact of chiral water clusters on optical rotation
accounts for the sudden shift in the specific rotation of dilute solutions (less than 0.5%) of L-ascorbic acid in water, based on the D/H ratio. The
influence of the isotopic composition of water was confirmed by studying the temperature-dependent mutarotation kinetics of D-glucose and L-and
D-galactose in Arrhenius coordinates.
The mutarotation process in natural high-resistivity water is characterized by an activation energy (Ea) of 40.8±1.4 kJ mol
-1
, while in deuterium-
depleted water, Ea = 63.6±3.5 kJ mol
-1
. This results in a kinetic isotope effect for deuterium (KIED) of 1.6.
Conclusion: Methodological approaches have been developed to control chiral switching based on the isotopic composition of water in vivo and in
vitro. The study of changes in the optical activity of hierarchical structures in the human body, the influence of solvent properties on the
mechanisms of optical rotation, as well as the use of KIED values, can be utilized to monitor various chiral transitions in vitro and living organisms.
Keywords: Kinetic isotope effect, Deuterium/protium ratio, Chiral switching
© 2024 The Authors. Published by Innovare Academic Sciences Pvt Ltd. This is an open access article under the CC BY license (https://creativecommons.org/licenses/by/4.0/)
DOI: https://dx.doi.org/10.22159/ijap.2024v16i3.50481 Journal homepage: https://innovareacademics.in/journals/index.php/ijap
INTRODUCTION
The renowned J.-B. Biot established the principles of dynamic
stereochemistry [1], which explain various processes involving
optically active compounds. The term "chiral switch" was first used to
refer to the extraction of the active enantiomer from a racemate or
mixture of diastereoisomers (epimers) patented as drugs [2]. Later,
this term began to be used for the synthesis of new enantiomers of
pharmaceutical substances that had not previously been used as drugs
[3]. The stereochemical properties of drug enantiomers contribute to
differences in pharmacokinetic and pharmacological profiles, as well
as the ways they interact with chiral biological targets [4]. The use of a
single pure enantiomer instead of a racemate improves the
effectiveness and/or safety of treatment [5] and promotes the
development of new drugs across various pharmacological classes [6].
The significance of chiral switching extends beyond the
development and production of enantiopure drugs. This concept
has significantly expanded in scope. Over the past decades,
scientific knowledge has accumulated regarding the change in the
chirality of drugs during biotransformation (stereoselective
metabolism), leading to the formation of numerous optically active
products with unknown properties [7, 8]. These degradation
products can interact with the naturally occurring alternating
hierarchical structures in the body [9].
Changes in the pharmacokinetic properties of chiral compounds
are observed at molecular, cellular, and organismal levels (fig. 1).
For example, deuterated drugs are new compounds in which
protium (H) atoms are replaced by deuterium (D) atoms [10]. The
kinetic isotope effect of deuterium (KIED) results in a reduction in
the drug's dosage and toxicity and also prevents the epimerization
of optically active substances. Dose-response diagrams for a
unicellular organism demonstrate the importance of deuterium as
an essential trace element. Deficiency or excess of this element can
reduce the organism's vitality. The homeostasis area is tightly
regulated by the ratio of deuterium to hydrogen at various
temperatures [11]. Another example that highlights the
significance of broadening the concept of "chiral switching" is the
shift in the direction of optical rotation that occurs as hierarchical
structures develop in living systems. This makes it possible to use
chirality as a tool for the stratification of hierarchical systems in
living organisms and non-living objects [12, 13].
Chiral switching occurs during the process of inducing chirality in
achiral molecules and giant heterogeneous water clusters [14],
facilitated by small optically active structures known as "sergeant-
soldier" [15]. The accumulated experimental data necessitate the
generalization and development of new approaches to control chiral
switching based on the kinetic isotope effect of deuterium [16, 17].
Deuterium is one of the essential elements [18]. Its main role in
living organisms and laboratory settings is to participate in chiral
switching at different hierarchical levels within the body. The
presence of deuterium (D) in a drug molecule or solvent, in various
ratios with protium (H), enables the control of various types of chiral
switching. The behavior of optically active compounds from various
chemical classes (such as the amino acid valine, ascorbic acid, and
carbohydrates like glucose and galactose) in waters with different
deuterium/protium ratios is discussed.
International Journal of Applied Pharmaceutics
ISSN-0975-7058 Vol 16, Issue 3, 2024