Vol.:(0123456789) 1 3
Journal of Radioanalytical and Nuclear Chemistry
https://doi.org/10.1007/s10967-019-06826-w
Measurement of neutron dose from p+
181
Ta reaction at different
proton energies via LET spectrometry
G. S. Sahoo
1
· S. P. Tripathy
1,3
· S. Paul
1
· S. C. Sharma
2
· D. S. Joshi
1
· T. Bandyopadhyay
1,3
· M. S. Kulkarni
1,3
Received: 25 March 2019
© Akadémiai Kiadó, Budapest, Hungary 2019
Abstract
While measuring the neutron dose in accelerator radiation environment using CR-39 detector for radiation protection purpose,
LET (linear energy transfer) spectrometry method is implemented when the information about the radiation source term is
unknown. In this work, the neutron dose has been measured for p+
181
Ta reaction at different proton energies i.e. 8–20 MeV
by LET spectrometry method using CR-39 detectors. The track density in CR-39 was found to increase exponentially with
the proton energy and an empirical relation has been established. The dosimetric quantities viz. absorbed dose (D
LET
) and
dose equivalent (H
LET
) were determined from the LET spectra and both these quantities were found to be increasing with
the proton energy. Empirical relations were generated, which will be useful for predicting dose in similar radiation environ-
ment. The dosimetric data generated in this study would be useful for radiation protection of occupational workers working
in the accelerator radiation environment.
Keywords LET spectrometry · Neutron dosimetry · CR-39 detector · p+
181
Ta reaction · Dose equivalent
Introduction
The radiological risk from ionizing radiation depends on
both the quantity and the quality of the radiation. The radia-
tion quantity is the measure of the absorbed dose by the
primary as well as the secondary ionizing radiation whereas
the radiation quality is best understood by the procedures of
microdosimetry where the spatial distribution of the energy
deposition plays the major role. The well known instrument
for the practice of microdosimetry is TEPC (tissue equiva-
lent proportional counter) [1] which measures the distribu-
tion of lineal energy transfer. The major limitations of TEPC
lie in the domain of high dose rate and in the presence of
intense low LET (linear energy transfer) radiations. Hence,
LET spectrometer [2] based on SSNTD (solid state nuclear
track detector) has been developed which has advantage of
measuring the high LET particles in the presence of intense
low LET radiations. In the accelerator radiation environ-
ment, the presence of low LET gamma radiation makes the
neutron dosimetry complicated [3]. Hence the LET spec-
trometry method [4] by using CR-39 SSNTD is preferred as
it is insensitive to gamma radiation. This method does not
involve the complicated unfolding procedures [5] as needed
in case of energy spectrometry. Also this method is simple,
convenient and does not require the discrimination of differ-
ent radiation components.
LET spectrometry method for neutron dosimetry has
successfully been implemented for cosmic rays [6, 7], high
energy
12
C beams [8], mono-energetic neutrons [9], D–T
neutrons [10], neutrons produced in p+
9
Be, p+
12
C reactions
[11, 12] and in combination of
7
Li and
181
Ta target [13]. In
this work, the neutron dose has been measured for p+
181
Ta
reaction at different proton energies i.e. from 8 to 20 MeV
by LET spectrometry method. Although the p+
181
Ta reac-
tion has been studied earlier [14], the emphasis was given
on the determination of neutron spectrum (energy distribu-
tion) from the track parameters. However, in this work it is
focused on the determination of LET spectra for p+
181
Ta
reaction, without determining the energy spectrum. Tanta-
lum is often used in accelerator components such as beam
dump, target holder and other structural components and
* G. S. Sahoo
sahoo.gouri232@gmail.com
1
Health Physics Division, Bhabha Atomic Research Centre,
Mumbai, 400 085, India
2
Nuclear Physics Division, Bhabha Atomic Research Centre,
Mumbai, 400 085, India
3
Homi Bhabha National Institute, Anushaktinagar,
Mumbai 400 094, India