Introduction
Woodceramics are, in a sense, carbon/carbon hybrid
materials consisting of plant-originated amorphous
carbon reinforced by glassy carbon generated from
resin. They are higher in strength than wood, but lighter
and readily machinable as compared with ceramics [1].
They were originally prepared by carbonizing wood or
woody materials impregnated with thermosetting resin,
such as phenol resin, in a vacuum furnace [2]. Thus,
their potential for use as electromagnetic shielding
materials [3], lubricating materials [4, 5], and sensor
materials [6] has been reported.
Recently, woodceramics are considered environ-
ment benign materials or so-called ecomaterials,
because they can be produced from carbon-containing
industrial wastes and take part as a member of a closed
material recycle system, and their by-products, such as
the decomposition products, can be recycled [7]. For
instance, in the apple products industry in Aomori
Prefecture, Japan, about 4250 t/year of apple juice
extract residues, i.e., apple pomace, which corresponds
to about 20% of the raw material, is being wasted. Thus,
woodceramics were produced from apple pomace, and
detailed studies have been made on the effect of
sintering conditions as well as characterization of them,
such as densities, structures, and thermooxidative
properties for use as sorbents [8, 9].
Similarly, as Japanese enjoy more western dishes,
more eggs and chicken meat are consumed, and tradi-
tional farms are increasing scale to bring up poultries
and broilers, resulting in the production of larger
amount of chicken wastes (feces). It is reported that
such chicken wastes amounting to 8.1 million tons
from poultry and 5 million tons from other chickens
are being disposed annually. This is becoming a
serious problem also in US because, not only it lacks
proper means to dispose large amount of wastes, but
also such animal manure causes environmental
concerns such as polluting water [10] and delivering
unfavorable odor that annoy people.
As a measure for coping with this problem, it had
long been proposed to use chicken wastes as agricultural
fertilizers, since chicken feces contain elements and
compounds such as calcium, potassium, nitrogen,
magnesium, and the like in addition to carbon. This
proposal is ideal in that the wastes can be used in a
closed cycle in the farm sites. However, the chicken
wastes or carbonized products obtained therefrom were
found to have strong unfavorable smell, which was
found as a serious problem to be overcome.
Thus, woodceramics using chicken wastes free
from odor was characterized by X-ray diffraction
(XRD) and thermal analysis. The chemical composi-
tion of carbonized chicken waste and woodceramics
made from chicken waste (CH800) was determined by
X-ray fluorescence spectroscopy (SQX). The reason
why they are odor-free was investigated by mainly
using simultaneous thermogravimetry-differential
thermal analysis (TG-DTA) coupled with evolved gas
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© 2005 Akadémiai Kiadó, Budapest Springer, Dordrecht, The Netherlands
Journal of Thermal Analysis and Calorimetry, Vol. 80 (2005) 489–493
TG-DTA/GC-MS STUDY OF ODORLESS WOODCERAMICS FROM
CHICKEN WASTES
R. Ozao
1*
, T. Okabe
2
, T. Arii
3
, Y. Nishimoto
4
, Y. Cao
5
, N. Whitely
5
and W.-P. Pan
5
1
SONY Institute of Higher Education, Atsugi, 243-8501 Kanagawa, Japan
2
Aomori Industrial Research Center, Environmental Technology Div., 4-11-6, Daini-tonyamachi, 030-0113 Aomori, Japan
3
Rigaku Corporation, 3-9-12 Matsubara, Akishima, 196-8666 Tokyo, Japan
4
Kanagawa University, Dept. of Chemistry, Hiratsuka, 259-1295 Kanagawa, Japan
5
Western Kentucky University, Dept. of Chemistry, 1 Big Red Way, Bowling Green, KY, 42101, USA
An odorless woodceramics (CH800), which was prepared by carbonizing chicken wastes with phenolic resin, was characterized by
XRD and thermal analysis. CH800 was found to consist mainly of amorphous carbon (non-graphitizing carbon) as studied by XRD.
Differing from carbonized chicken waste, CH800 was completely free of unfavorable smell. The source of strong smell of carbonized
chicken waste was studied by using TG-DTA combined with EGA technique using gas chromatography and mass spectrometry
(TG-DTA/GC-MS). As a result, it was found that CH800 was completely free of compounds having strong smell, i.e., ethanol,
acetonitrile, pyridine, styrene, benzonitrile and benzofuran, whereas carbonized chicken waste contained all of these compounds.
Keywords: adsorption, chicken waste, ecomaterial, micropores, smell, sorbent, TG-DTA/GC-MS, woodceramics
* Author for correspondence: ozao@ei.shohoku.ac.jp