Vol.:(0123456789)
Euro-Mediterranean Journal for Environmental Integration
https://doi.org/10.1007/s41207-024-00467-6
ORIGINAL PAPER
Improving water security and sanitation in rural areas: comparative
evaluation of TiO
2
and photo‑Fenton processes for rural wastewater
treatment and reuse
Yasmin Cherni
1
· Djebali Kais
2
· Hamadi Kallali
1
· Mohamed Ali Wahab
1
· Samira Melki
1
· Jihene Tayahi
1
·
Isabel Oller
3
· Plakas Konstantinos
4
Received: 7 July 2023 / Accepted: 13 January 2024
© Springer Nature Switzerland AG 2024
Abstract
Wastewater treatment and reuse are essential for addressing water shortages and promoting sustainable water security and
sanitation development, particularly in rural areas. This paper aims to compare the performance of various oxidation pro-
cesses, including UV/photo-Fenton, solar photo-Fenton, solar photocatalysis using TiO
2
, and UV/TiO
2
, for treating rural
wastewater using response surface methodology (RSM). The effects of several factors on the photocatalytic treatment per-
formance in terms of reducing organic pollutants and disinfecting wastewater were evaluated using Plackett–Burman and
Box–Behnken experimental designs. The outcomes indicate that pH is a crucial factor for enhancing photocatalytic treatment
efficiency. By optimizing the photocatalytic treatment conditions, the Fenton process achieved the highest removal efficiencies
for different pollutants. Specifically, at a pH of 3, a concentration of 1.678 mg/L of the reagent Fe
2+
was sufficient to reduce
COD, TOC, and turbidity by 44.88, 55, and 97.21%, respectively, within just 1 h. Interestingly, the optimized conditions
led to significant removal of ammonium (69.74%). Bacteriological analyses further demonstrated reductions in total germs
and E. coli and the absence of streptococci. The effect of phytotoxicity on lettuce seed growth was evaluated in terms of the
germination index (GI). The treated wastewater showed no phytotoxic effects and achieved a GI above 99%. The findings
highlight the effectiveness of the Fenton process as a viable treatment alternative for enhancing effluent quality and increas-
ing the potential for the agricultural reuse of effluent as fertilizer.
Graphical abstract
Box Behnken design
&
Placke Burman
design
Phytotoxicity
test
Optimum conditions :
:3 ; Reaction time :60 min ; [Fe
2+
]:
1.678 mg/L
COD removal efficiency :44.88% ;
TOC removal efficiency : 55% ;
Turbidity removal efficiency : 97.21% ;
Ammonium removal efficiency :
69.74% ;
Reduction of pathogenic microorganisms
pH
Responsible Editor: Mohamed Ksibi.
Extended author information available on the last page of the article