Citation: Magadán-Corpas, P.;
Pérez-Valero, Á.; Ye, S.; Sordon, S.;
Huszcza, E.; Popło ´ nski, J.; Villar, C.J.;
Lombó, F. Gut Microbiota and
Inflammation Modulation in a Rat
Model for Ulcerative Colitis after the
Intraperitoneal Administration of
Apigenin, Luteolin, and Xanthohumol.
Int. J. Mol. Sci. 2024, 25, 3236.
https://doi.org/10.3390/ijms25063236
Academic Editors: Fernando
Santos-Beneit and Rustam I. Aminov
Received: 24 January 2024
Revised: 5 March 2024
Accepted: 8 March 2024
Published: 12 March 2024
Copyright: © 2024 by the authors.
Licensee MDPI, Basel, Switzerland.
This article is an open access article
distributed under the terms and
conditions of the Creative Commons
Attribution (CC BY) license (https://
creativecommons.org/licenses/by/
4.0/).
International Journal of
Molecular Sciences
Article
Gut Microbiota and Inflammation Modulation in a Rat Model for
Ulcerative Colitis after the Intraperitoneal Administration of
Apigenin, Luteolin, and Xanthohumol
Patricia Magadán-Corpas
1,2,3
, Álvaro Pérez-Valero
1,2,3
, Suhui Ye
1,2,3
, Sandra Sordon
4
, Ewa Huszcza
4
,
Jarosław Popło ´ nski
4
, Claudio J. Villar
1,2,3
and Felipe Lombó
1,2,3,
*
1
Research Group BIONUC (Biotechnology of Nutraceuticals and Bioactive Compounds), Departamento de
Biología Funcional, Área de Microbiología, Universidad de Oviedo, 33006 Oviedo, Spain;
magadanpatricia@uniovi.es (P.M.-C.); apv.moratalla@gmail.com (Á.P.-V.); yesuhui@uniovi.es (S.Y.);
cjvg@uniovi.es (C.J.V.)
2
IUOPA (Instituto Universitario de Oncología del Principado de Asturias), 33006 Oviedo, Spain
3
ISPA (Instituto de Investigación Sanitaria del Principado de Asturias), 33006 Oviedo, Spain
4
Department of Food Chemistry and Biocatalysis, Wrocław University of Environmental and Life Sciences,
Norwida 25, 50-375 Wrocław, Poland; sandra.sordon@upwr.edu.pl (S.S.); ewa.huszcza@upwr.edu.pl (E.H.);
jaroslaw.poplonski@upwr.edu.pl (J.P.)
* Correspondence: lombofelipe@uniovi.es; Tel.: +34-985103593
Abstract: Ulcerative colitis (UC) is a chronic inflammatory disorder affecting the colon, with symp-
tomatology influenced by factors including environmental, genomic, microbial, and immunological
interactions. Gut microbiota dysbiosis, characterized by bacterial population alterations, contributes
to intestinal homeostasis disruption and aberrant immune system activation, thereby exacerbating
the inflammatory state. This study assesses the therapeutic efficacy of intraperitoneal (IP) injected
flavonoids (apigenin, luteolin, and xanthohumol) in the reduction of inflammatory parameters and
the modulation of the gut microbiota in a murine model of ulcerative colitis. Flavonoids interact
with gut microbiota by modulating their composition and serving as substrates for the fermentation
into other anti-inflammatory bioactive compounds. Our results demonstrate the effectiveness of
luteolin and xanthohumol treatment in enhancing the relative abundance of anti-inflammatory mi-
croorganisms, thereby attenuating pro-inflammatory species. Moreover, all three flavonoids exhibit
efficacy in the reduction of pro-inflammatory cytokine levels, with luteolin strongly demonstrating
utility in alleviating associated physical UC symptoms. This suggests that this molecule is a potential
alternative or co-therapy to conventional pharmacological interventions, potentially mitigating their
adverse effects. A limited impact on microbiota is observed with apigenin, and this is attributed
to its solubility constraints via the chosen administration route, resulting in its accumulation in
the mesentery.
Keywords: inflammatory bowel disease; gut microbiota; flavonoid; anti-inflammatory
1. Introduction
Inflammatory bowel disease (IBD) is a term that encompasses two conditions, Crohn’s
disease (CD) and ulcerative colitis (UC), both characterized by chronic inflammation
of the gastrointestinal tract. While CD can affect any part of the intestinal tract (from
mouth to anus), UC only affects the colon, causing abdominal pain, mucus, diarrhea, and
blood stool [1]. IBD represents a group of archetypal complex disorders distinguished by
chronic and varied symptoms, influenced by the interplay among environmental, genomic,
microbial, and immunological factors [2].
Multiple investigations have corroborated notable distinctions in the composition,
diversity, and/or abundance of gut microbiota (dysbiosis) between healthy individuals
and those with IBD, leading to the loss of intestinal homeostasis or improper immune
Int. J. Mol. Sci. 2024, 25, 3236. https://doi.org/10.3390/ijms25063236 https://www.mdpi.com/journal/ijms