Temperature dependence measurements of the supercurrent-phase relationship in niobium nanobridges A. G. P. Troeman, 1 S. H. W. van der Ploeg, 2 E. Il’Ichev, 2 H.-G. Meyer, 2 A. A. Golubov, 1 M. Yu. Kupriyanov, 3 and H. Hilgenkamp 1 1 Faculty of Science and Technology and Mesa + Institute for Nanotechnology, University of Twente, P.O. Box 217, 7500 AE Enschede, The Netherlands 2 Department of Cryoelectronics, Institute for Photonic Technology, D-07702 Jena, Germany 3 Nuclear Physics Institute, Moscow State University, 119992 Moscow, Russia Received 16 August 2007; published 14 January 2008 The current-phase relationship has been measured as a function of temperature for niobium nanobridges with different widths. A deformation from Josephson-like sinusoidal characteristics at high temperatures to sawtooth shaped curves at intermediate and multivalued relationships at low temperatures was observed. Based on this, possible hysteresis in the current-voltage characteristics of niobium nanobridge superconducting quantum interference devices can be attributed to phase slippage. DOI: 10.1103/PhysRevB.77.024509 PACS numbers: 74.78.Na, 74.45.c, 74.50.r, 85.25.Cp I. INTRODUCTION One of the fundamental characteristics of superconducting structures is the relationship between the supercurrent through and the phase difference across the structure. The prediction 1 and first experimental verification 2 of periodical current-phase relationships CPRsin superconductor- insulator-superconductor tunnel junctions triggered the onset of research on Josephson devices. Much of the classical stud- ies on this subject focused on structures where two supercon- ducting layers are separated by a barrier with a thickness of the order of the superconducting coherence length . With the advances in nanotechnology, the development of super- conducting structures with lateral dimensions of the order of also became possible. Examples of such systems are super- conducting nanobridges, which, when of sufficiently small dimensions, are known to exhibit a periodical CPR. 3,4 Based on this similarity to classical Josephson tunnel junctions, the development of superconducting quantum interference de- vices SQUIDsincorporating two of such nanobridges has been a topic of ongoing research, e.g., for the detection of the magnetization reversal of small magnetic clusters 57 and in scanning SQUID microscopes. 811 The application of super- conducting nanobridges as single photon detectors, for in- stance, as described in Ref. 12, has been a topic of interest in recent years. In addition, hot electron bolometers based on superconducting nanobridges are explored as detectors in as- trophysical observations at terahertz frequencies. 13 Recent fundamental interest in superconducting nanobridges has fur- thermore been motivated by the possible application of such structures in flux qubits. 14,15 Even though applications based on the Josephson-like characteristics of superconducting nanobridges have been in- vestigated extensively, up until now, the exact nature of the CPRs in these structures has mainly been studied theoreti- cally. It is predicted to be dependent on the dimensions of the structure. According to the Kulik-Omelyanchuk model, 16 a gradual temperature Tdependent deformation of the CPR from sinusoidal at high T to sawtoothlike at lower T is ex- pected in the clean limit. Strongly nonsinusoidal CPRs at low T are also predicted in the diffusive regime for nano- wires with lengths L 0 l 1/2 where 0 is the BCS coher- ence length and l the electronic mean free pathand small transverse sizes W L. These models were qualitatively veri- fied for the CPR in clean ballistic niobium point contacts. 17 Recent quantitative agreement between experiment and theory was reported for aluminum atomic contacts. 18 Likharev and Yakobson first considered the effect of an in- creasing weak link length on the CPR for structures in which the temperature is close to the critical temperatures of both the electrodes T c and the nanobridge T c . 19 Their model describes a similar deformation of the CPR, from sinusoidal to sawtoothlike, as a function of increasing bridge length. Furthermore, at a critical length L 3.5 0 T, with 0 Tthe Ginzburg-Landau GLcoherence length, the nature of the CPR becomes multivalued. In this limit, superconductivity is suppressed above the critical current by phase slippage of the superconducting order parameter in the structure. Dur- ing a phase slip, the order parameter fluctuates to zero, al- lowing the relative phase to relax by 2and resulting in a voltage pulse. In the GL regime, this model was extended to two dimensions in Ref. 20. For wide a 3.5T and long L 4.4T nanobridges, the coherent motion of vortices across the structure is expected to determine the CPR. For fixed values of the bridge length and T c = T c , the de- scribed deformation of the CPR and crossover as a function of decreasing temperature were discussed quantitatively by Kupriyanov et al. 21 within a model valid at arbitrary tem- peratures. In terms of the GL approach, this can be explained by the fact that Tincreases as a function of temperature, which, for fixed L, is physically similar to a decrease of the effective bridge length. Based on the models discussed above, the predicted transition of the CPR in a superconduct- ing nanobridge L 0 l 1/2 is qualitatively depicted in Fig. 1. The dotted line corresponds to the sharp drop in phase related to the phase slip mechanism. Previously, the described crossover was studied only in- directly in experiment by measuring the power dependence of Shapiro steps in the current-voltage IVcurves of microwave-irradiated Sn microbridges. 22 This study con- PHYSICAL REVIEW B 77, 024509 2008 1098-0121/2008/772/0245095©2008 The American Physical Society 024509-1